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000051542 0247_ $$2DOI$$a10.1103/PhysRevB.72.094104
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000051542 084__ $$2WoS$$aPhysics, Condensed Matter
000051542 1001_ $$0P:(DE-HGF)0$$aStephens, P.$$b0
000051542 245__ $$aHigh-pressure diffraction studies on Ca2RuO4
000051542 260__ $$aCollege Park, Md.$$bAPS$$c2005
000051542 300__ $$a094104-1 - 094104-7
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000051542 440_0 $$04919$$aPhysical Review B$$v72$$x1098-0121
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000051542 520__ $$aWe studied the crystal and magnetic structure of Ca2RuO4 as function of pressure with different diffraction techniques. The first-order phase transition observed at a moderate pressure of P=0.5 GPa between the insulating and the metallic high-pressure phase is characterized by a broad region of phase coexistence. The following structural changes are observed as function of pressure: (a) A discontinuous change of both the tilt and rotational angle of the RuO6-octahedra at this transition, (b) a gradual decrease of the tilt angle in the high-pressure phase (P>0.5 GPa), and (c) the disappearance of the tilt above 5.5 GPa leading to a higher symmetry structure. The magnetism was studied by single-crystal neutron diffraction: The ferromagnetic component of the high-pressure phase and a rearrangement of antiferromagnetic order in the low-pressure phase have been observed.
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000051542 7001_ $$0P:(DE-HGF)0$$aFriedt, O.$$b1
000051542 7001_ $$0P:(DE-HGF)0$$aMarshall, W. G.$$b2
000051542 7001_ $$0P:(DE-Juel1)VDB1436$$aSchmidt, W.$$b3$$uFZJ
000051542 7001_ $$0P:(DE-HGF)0$$aNakamura, F.$$b4
000051542 7001_ $$0P:(DE-HGF)0$$aNakatsuji, S.$$b5
000051542 7001_ $$0P:(DE-HGF)0$$aMaeno, Y.$$b6
000051542 7001_ $$0P:(DE-HGF)0$$aLengssdorf, R.$$b7
000051542 7001_ $$0P:(DE-HGF)0$$aAbd-Elmeguid, M. M.$$b8
000051542 7001_ $$0P:(DE-HGF)0$$aBraden, M.$$b9
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000051542 8567_ $$uhttp://hdl.handle.net/2128/1153$$uhttp://dx.doi.org/10.1103/PhysRevB.72.094104
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