TY - JOUR AU - Stephens, P. AU - Friedt, O. AU - Marshall, W. G. AU - Schmidt, W. AU - Nakamura, F. AU - Nakatsuji, S. AU - Maeno, Y. AU - Lengssdorf, R. AU - Abd-Elmeguid, M. M. AU - Braden, M. TI - High-pressure diffraction studies on Ca2RuO4 JO - Physical review / B VL - 72 IS - 9 SN - 1098-0121 CY - College Park, Md. PB - APS M1 - PreJuSER-51542 SP - 094104 PY - 2005 N1 - Record converted from VDB: 12.11.2012 AB - We studied the crystal and magnetic structure of Ca2RuO4 as function of pressure with different diffraction techniques. The first-order phase transition observed at a moderate pressure of P=0.5 GPa between the insulating and the metallic high-pressure phase is characterized by a broad region of phase coexistence. The following structural changes are observed as function of pressure: (a) A discontinuous change of both the tilt and rotational angle of the RuO6-octahedra at this transition, (b) a gradual decrease of the tilt angle in the high-pressure phase (P>0.5 GPa), and (c) the disappearance of the tilt above 5.5 GPa leading to a higher symmetry structure. The magnetism was studied by single-crystal neutron diffraction: The ferromagnetic component of the high-pressure phase and a rearrangement of antiferromagnetic order in the low-pressure phase have been observed. KW - J (WoSType) LB - PUB:(DE-HGF)16 UR - <Go to ISI:>//WOS:000232228500033 DO - DOI:10.1103/PhysRevB.72.094104 UR - https://juser.fz-juelich.de/record/51542 ER -