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@ARTICLE{Hpfner:51779,
author = {Höpfner, M. and Luo, B. P. and Massoli, P. and Cairo, F.
and Spang, R. and Snels, M. and Di Donfrancesco, G. and
Stiller, G. and von Clarmann, T. and Fischer, H. and
Biermann, U.},
title = {{S}pectroscopic evidence for {NAT}, {STS}, and ice in
{MIPAS} infrared limb emission measurements of polar
stratospheric clouds},
journal = {Atmospheric chemistry and physics},
volume = {6},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-51779},
pages = {1201 - 1219},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {We have analyzed mid-infrared limb-emission measurements of
polar stratospheric clouds ( PSCs) by the Michelson
Interferometer for Passive Atmospheric Sounding ( MIPAS)
during the Antarctic winter 2003 with respect to PSC
composition. Coincident Lidar observations from McMurdo were
used for comparison with PSC types 1a, 1b and 2. Application
of new refractive index data of beta-NAT have allowed to
accurately simulate the prominent spectral band at 820
cm(-1) observed by MIPAS at the location where the Lidar
instrument observed type 1a PSCs. Broadband spectral fits
covering the range from 780 to 960 cm(-1) and from 1220 to
1490 cm(-1) showed best agreement with the MIPAS
measurements when spectroscopic data of NAT were used to
simulate the MIPAS spectra. MIPAS measurements collocated
with Lidar observations of Type 1b and Type 2 PSCs could
only be reproduced by assuming a composition of supercooled
ternary H2SO4/HNO3/H2O solution ( STS) and of ice,
respectively. Particle radius and number density profiles
derived from MIPAS were generally consistent with the Lidar
observations. Only in the case of ice clouds, PSC volumes
are partly underestimated by MIPAS due to large cloud
optical thickness in the limb-direction. A comparison of
MIPAS cloud composition and Lidar PSC-type determination
based on all available MIPAS-Lidar coincident measurements
revealed good agreement between PSC-types 1a, 1b and 2, and
NAT, STS and ice, respectively. We could not find
spectroscopic evidence for the presence of nitric acid
dihydrate ( NAD) from MIPAS observations of PSCs over
Antarctica in 2003.},
keywords = {J (WoSType)},
cin = {ICG-I},
ddc = {550},
cid = {I:(DE-Juel1)VDB47},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000236950100001},
url = {https://juser.fz-juelich.de/record/51779},
}