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@ARTICLE{Bossmeyer:52213,
author = {Bossmeyer, J. and Brauers, T. and Richter, C. and Rohrer,
F. and Wegener, R. and Wahner, A.},
title = {{S}imulation {C}hamber {S}tudies on the {NO}3 {C}hemistry
of {A}tmospheric {A}ldehydes},
journal = {Geophysical research letters},
volume = {33},
issn = {0094-8276},
address = {Washington, DC},
publisher = {American Geophysical Union},
reportid = {PreJuSER-52213},
pages = {L18810},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {Absolute reaction rate studies of NO3 radicals with 4
aldehydes were performed in the atmosphere simulation
chamber SAPHIR at the Research Center Julich. Rate
coefficients ( ethanal: 2.6 +/- 0.5, propanal: 5.8 +/- 1.0,
butanal: 11.9 +/- 1.4, benzaldehyde: 2.2 +/- 0.6; in 10(-15)
cm(3) s(-1) at 300 K) were determined from measured
concentration time profiles of aldehydes and NO3 at near
ambient conditions. The values for the aliphatic aldehydes
are in good agreement with the most recent recommendations (
IUPAC Subcommittee on Gas Kinetic Data Evaluation for
Atmospheric Chemistry: Evaluated kinetic and photochemical
data for atmospheric chemistry, 2005, available at http://
www. iupac- kinetic. ch. cam. ac. uk). The measured
concentration- time profiles of precursor aldehydes, NO3,
NO2, and of product aldehydes were compared to model
calculations based on the MCM v3 ( Jenkin et al., 2003;
Saunders et al., 2003). Differences between measurements and
model are attributed to a major interference of the GC
system to peroxyacyl nitrates. In addition modifications to
the rate constants in the MCM are suggested.},
keywords = {J (WoSType)},
cin = {ICG-II / JARA-ENERGY},
ddc = {550},
cid = {I:(DE-Juel1)VDB48 / $I:(DE-82)080011_20140620$},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Geosciences, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000240943400002},
doi = {10.1029/2006GL026778},
url = {https://juser.fz-juelich.de/record/52213},
}