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@ARTICLE{Lagarde:52843,
author = {Lagarde, F. and Pütz, T. and Dressel, J. and Führ, F.},
title = {{S}imultaneous {D}etermination of {E}thidimuron,
{M}ethabenzthiazuron, and {T}heir {T}wo {M}ajor
{D}egradation {P}roducts in {S}oil},
journal = {Journal of agricultural and food chemistry},
volume = {54},
issn = {0021-8561},
address = {Washington, DC [u.a.]},
publisher = {American Chemical Society (ACS)},
reportid = {PreJuSER-52843},
pages = {7450 - 7459},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {An analytical method has been developed for the
quantification of two herbicides (ethidimuron and
methabenzthiazuron) and their two main soil derivatives.
This method involves fluidized-bed extraction (FBE) prior to
cleanup and analysis by reverse-phase liquid chromatography
with UV detection at 282 nm. FBE conditions were established
to provide efficient extraction without degradation of the
four analytes. (14)C-labeled compounds were used for the
optimization of extraction and purification steps and for
the determination of related efficiencies. Extraction was
optimal using a fexIKA extractor operating at 110 degrees C
for three cycles (total time = 95 min) with 75 g of soil and
150 mL of a 60:40 v/v acetone/water mixture. Extracts were
further purified on a 500 mg silica SPE cartridge.
Separation was performed on a C18 Purosphere column (250 mm
x 4 mm i.d.), at 0.8 mL min(-1) and 30 degrees C with an
elution gradient made up of phosphoric acid aqueous solution
(pH 2.2) and acetonitrile. Calibration curves were found to
be linear in the 0.5-50 mg L(-1) concentration range.
Besides freshly spiked soil samples, method validation
included the analysis of samples with aged residues.
Recovery values, determined from spiked samples, were close
to $100\%.$ Limits of detection ranged between 2 and 3
microg kg(-1) of dry soil and limits of quantification
between 8 and 10 microg kg(-1) of dry soil. An attempt to
improve these performances by using fluorescence detection
following postcolumn derivatization by
orthophthalaldehyde-mercaptoethanol reagent was
unsuccessful.},
keywords = {Benzothiazoles: analysis / Benzothiazoles: chemistry /
Chromatography, High Pressure Liquid: methods / Herbicides:
analysis / Methylurea Compounds: analysis / Methylurea
Compounds: chemistry / Photolysis / Sensitivity and
Specificity / Soil: analysis / Solutions / Benzothiazoles
(NLM Chemicals) / Herbicides (NLM Chemicals) / Methylurea
Compounds (NLM Chemicals) / Soil (NLM Chemicals) / Solutions
(NLM Chemicals) / ethidimuron (NLM Chemicals) /
methabenzthiazuron (NLM Chemicals) / J (WoSType)},
cin = {ICG-IV},
ddc = {630},
cid = {I:(DE-Juel1)VDB50},
pnm = {Terrestrische Umwelt},
pid = {G:(DE-Juel1)FUEK407},
shelfmark = {Agriculture, Multidisciplinary / Chemistry, Applied / Food
Science $\&$ Technology},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:17002407},
UT = {WOS:000240795400007},
doi = {10.1021/jf061042v},
url = {https://juser.fz-juelich.de/record/52843},
}