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000052925 0247_ $$2DOI$$a10.1146/annurev.physchem.58.032806.104432
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000052925 084__ $$2WoS$$aChemistry, Physical
000052925 1001_ $$0P:(DE-HGF)0$$aRudich, Y.$$b0
000052925 245__ $$aAging of organic aerosols: bridging the gap between laboratory and field studies
000052925 260__ $$aPalo Alto, Calif. [u.a.]$$bAnnual Reviews$$c2007
000052925 300__ $$a321 - 352
000052925 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
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000052925 440_0 $$015801$$aAnnual Review of Physical Chemistry$$v58$$x0066-426X
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000052925 520__ $$aThe oxidation of organics in aerosol particles affects the physical properties of aerosols through a process known as aging. Atmospheric particles compose a huge set of specific organic compounds, most of which have not been identified in field measurements. Laboratory experiments inevitably address model systems of reduced complexity to isolate critical chemical phenomena, but growing evidence suggests that composition effects may play a central role in the atmospheric aging of organic particles. In this review we seek to address the connections between recent laboratory studies and recent field campaigns addressing the aging of organic aerosols. We review laboratory studies on the uptake of oxidants, the evolution of particle-water interactions, and the evolution of particle density with aging. Finally, we review field data addressing condensed-phase lifetimes of organic tracers. These data suggest that although matrix effects identified in the laboratory have taken a step toward reconciling laboratory-field disagreements, further work is needed to understand the actual aging rates of organics in ambient particles.
000052925 536__ $$0G:(DE-Juel1)FUEK406$$2G:(DE-HGF)$$aAtmosphäre und Klima$$cP22$$x0
000052925 588__ $$aDataset connected to Web of Science, Pubmed
000052925 650_2 $$2MeSH$$aAerosols: chemistry
000052925 650_2 $$2MeSH$$aOrganic Chemicals: chemistry
000052925 650_2 $$2MeSH$$aOxidation-Reduction
000052925 650_2 $$2MeSH$$aOzone: chemistry
000052925 650_2 $$2MeSH$$aResearch: methods
000052925 650_2 $$2MeSH$$aTime Factors
000052925 650_7 $$00$$2NLM Chemicals$$aAerosols
000052925 650_7 $$00$$2NLM Chemicals$$aOrganic Chemicals
000052925 650_7 $$010028-15-6$$2NLM Chemicals$$aOzone
000052925 650_7 $$2WoSType$$aJ
000052925 65320 $$2Author$$aheterogeneous atmospheric processes
000052925 65320 $$2Author$$ahygroscopic properties
000052925 65320 $$2Author$$asecondary organic aerosol
000052925 65320 $$2Author$$aoligomerization
000052925 65320 $$2Author$$arelative kinetics
000052925 65320 $$2Author$$achemical mechanisms
000052925 7001_ $$0P:(DE-HGF)0$$aDonahue, N.$$b1
000052925 7001_ $$0P:(DE-Juel1)16346$$aMentel, T. F.$$b2$$uFZJ
000052925 773__ $$0PERI:(DE-600)1470474-2$$a10.1146/annurev.physchem.58.032806.104432$$gVol. 58, p. 321 - 352$$p321 - 352$$q58<321 - 352$$tAnnual review of physical chemistry$$v58$$x0066-426X$$y2007
000052925 8567_ $$uhttp://dx.doi.org/10.1146/annurev.physchem.58.032806.104432
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