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@ARTICLE{Rudich:52925,
      author       = {Rudich, Y. and Donahue, N. and Mentel, T. F.},
      title        = {{A}ging of organic aerosols: bridging the gap between
                      laboratory and field studies},
      journal      = {Annual review of physical chemistry},
      volume       = {58},
      issn         = {0066-426X},
      address      = {Palo Alto, Calif. [u.a.]},
      publisher    = {Annual Reviews},
      reportid     = {PreJuSER-52925},
      pages        = {321 - 352},
      year         = {2007},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The oxidation of organics in aerosol particles affects the
                      physical properties of aerosols through a process known as
                      aging. Atmospheric particles compose a huge set of specific
                      organic compounds, most of which have not been identified in
                      field measurements. Laboratory experiments inevitably
                      address model systems of reduced complexity to isolate
                      critical chemical phenomena, but growing evidence suggests
                      that composition effects may play a central role in the
                      atmospheric aging of organic particles. In this review we
                      seek to address the connections between recent laboratory
                      studies and recent field campaigns addressing the aging of
                      organic aerosols. We review laboratory studies on the uptake
                      of oxidants, the evolution of particle-water interactions,
                      and the evolution of particle density with aging. Finally,
                      we review field data addressing condensed-phase lifetimes of
                      organic tracers. These data suggest that although matrix
                      effects identified in the laboratory have taken a step
                      toward reconciling laboratory-field disagreements, further
                      work is needed to understand the actual aging rates of
                      organics in ambient particles.},
      keywords     = {Aerosols: chemistry / Organic Chemicals: chemistry /
                      Oxidation-Reduction / Ozone: chemistry / Research: methods /
                      Time Factors / Aerosols (NLM Chemicals) / Organic Chemicals
                      (NLM Chemicals) / Ozone (NLM Chemicals) / J (WoSType)},
      cin          = {ICG-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB791},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK406},
      shelfmark    = {Chemistry, Physical},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:17090227},
      UT           = {WOS:000246652300013},
      doi          = {10.1146/annurev.physchem.58.032806.104432},
      url          = {https://juser.fz-juelich.de/record/52925},
}