Home > Publications database > Complex Formation and Proton Transfer between Formic Acid and Water Adsorbed on Au(111) Surfaces under UHV Conditions > print

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024 7 _ |2 DOI
|a 10.1007/s00339-007-3926-8
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041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Materials Science, Multidisciplinary
084 _ _ |2 WoS
|a Physics, Applied
100 1 _ |a Kazempoor, M.
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|u FZJ
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245 _ _ |a Complex Formation and Proton Transfer between Formic Acid and Water Adsorbed on Au(111) Surfaces under UHV Conditions
260 _ _ |c 2007
|a Berlin
|b Springer
300 _ _ |a 435 - 441
336 7 _ |a Journal Article
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440 _ 0 |a Applied Physics A
|x 0947-8396
|0 560
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|v 87
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a The coadsorption of formic acid and water on Au(111) surfaces has been investigated by means of vibrational and photoelectron spectroscopy (HREELS, XPS). Formic acid adsorbs at 90 K molecularly with vibrational modes characteristic for flat lying zig-zag chains in the mono- and multilayer regime, like in solid formic acid. Annealing results in a complete desorption at 190 K. Sequential adsorption of formic acid and water at 90 K shows no significant chemical interaction. Upon annealing the coadsorbed layer to 140 K a hydrogen-bonded cyclic complex of formic acid with one water molecule could be identified using isotopically labelled adsorbates (D2O, (HCOOD)-C-13). Upon further annealing this complex decomposes leaving molecularly adsorbed formic acid on the surface at 160 K, accompanied by a proton exchange between formic acid and water.
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700 1 _ |a Pirug, G.
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856 7 _ |u http://dx.doi.org/10.1007/s00339-007-3926-8
909 C O |o oai:juser.fz-juelich.de:53334
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