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@ARTICLE{Winkler:54926,
      author       = {Winkler, R. G. and Keller, S. and Rädler, J. O.},
      title        = {{I}ntramolecular dynamics of linear macromolecules by
                      fluorescence correlation spectroscopy},
      journal      = {Physical review / E},
      volume       = {73},
      number       = {4},
      issn         = {1539-3755},
      address      = {College Park, Md.},
      publisher    = {APS},
      reportid     = {PreJuSER-54926},
      pages        = {041919},
      year         = {2006},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {A theoretical description of the dynamics of DNA molecules
                      and actin filaments in solution as measured experimentally
                      by fluorescence correlation spectroscopy is provided and
                      compared to recent experimental results. Particular
                      attention is paid to the contribution of the intramolecular
                      dynamics to the fluorescence correlation function. Using a
                      semiflexible chain model, a theoretical expression is
                      presented for the fluorescence correlation spectroscopy
                      correlation function. The dependence of this function on
                      various model parameters, such as chain length, persistence
                      length, and fluorescence label density, is discussed. Our
                      investigations show that the intramolecular dynamics
                      provides a significant contribution or even dominates the
                      correlation function as soon as the longest intramolecular
                      relaxation time significantly exceeds the shortest
                      experimentally accessible time. Correspondingly, the shape
                      of the correlation function changes considerably.
                      Approximate analytical expressions are provided, which are
                      in qualitative agreement with the exact theoretical
                      solutions as well as experimental results, for both DNA and
                      actin filaments. Our approach is in agreement with the
                      predictions of the Zimm model, in the limit of very flexible
                      polymers, as well as the predictions of semiflexible polymer
                      models with respect to the intramolecular dynamics in
                      solution.},
      keywords     = {J (WoSType)},
      cin          = {IFF-TH-II},
      ddc          = {530},
      cid          = {I:(DE-Juel1)VDB31},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK414},
      shelfmark    = {Physics, Fluids $\&$ Plasmas / Physics, Mathematical},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000237146400076},
      doi          = {10.1103/PhysRevE.73.041919},
      url          = {https://juser.fz-juelich.de/record/54926},
}