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@ARTICLE{Shiratori:55901,
author = {Shiratori, Y. and Magrez, A. and Dornseiffer, J. and
Haegel, F.-H. and Pithan, C. and Waser, R.},
title = {{P}olymorphism in micro-, submicro-, and nanocrystalline
{N}a{N}b{O}3},
journal = {The journal of physical chemistry / B},
volume = {109},
issn = {1520-6106},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PreJuSER-55901},
pages = {20122 - 20130},
year = {2005},
note = {Record converted from VDB: 12.11.2012},
abstract = {NaNbO(3) powders with various particle sizes (ranging from
30 nm to several microns) and well-controlled stoichiometry
were obtained through microemulsion-mediated synthesis. The
effect of particle size on the phase transformation of the
prepared NaNbO(3) powders was studied using X-ray powder
diffraction, Raman spectroscopy, and nuclear site group
analysis based on these spectroscopic data. Coarsened
particles exhibit an orthorhombic Pbcm (D(2h)(11), no. 57)
structure corresponding to the bulk structure, as observed
for single crystals or powders prepared by conventional
solid-state reaction. The crystal symmetry of submicron
powders was refined with the space group Pmc2(1) (C(2v)(2),
no. 26). The reduced perovskite cell volumes of these
submicron powders were most expanded compared to all the
other structures. Fine particles with a diameter of less
than 70 nm as measured from SEM observations showed an
orthorhombic Pmma (D(2h)(5), no. 51) crystal symmetry. The
perovskite formula cell of this structure was pseudocubic
and was the most compact one. A possible mechanism of the
phase transformation is suggested.},
cin = {IFF-IEM / ICG-II},
ddc = {530},
cid = {I:(DE-Juel1)VDB321 / I:(DE-Juel1)VDB48},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:16853601},
UT = {WOS:000232959800012},
doi = {10.1021/jp052974p},
url = {https://juser.fz-juelich.de/record/55901},
}