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@ARTICLE{Dhont:56003,
      author       = {Dhont, J. K. G. and Wiegand, S. and Duhr, S. and Braun, D.},
      title        = {{T}hermodiffusion of {C}harged {C}olloids:
                      {S}ingle-{P}article {D}iffusion},
      journal      = {Langmuir},
      volume       = {23},
      issn         = {0743-7463},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {PreJuSER-56003},
      pages        = {1674 - 1683},
      year         = {2007},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {An expression for the single-particle thermal diffusion
                      coefficient of a charged colloidal sphere is derived on the
                      basis of force balance on the Brownian time scale in
                      combination with thermodynamics. It is shown that the
                      single-particle thermal diffusion coefficient is related to
                      the temperature dependence of the reversible work necessary
                      to build the colloidal particle, including the core, the
                      solvation layer, and the electrical double layer. From this
                      general expression, an explicit expression for the
                      contribution of the electrical double layer to the
                      single-particle thermal diffusion coefficient is derived in
                      terms of the surface charge density of the colloidal sphere,
                      the electrostatic screening length, and its core radius, to
                      within the Debye-Hückel approximation. This result is shown
                      to explain experimental data, for both thin and thick double
                      layers. In addition, a comparison with other theories is
                      made.},
      keywords     = {J (WoSType)},
      cin          = {IFF-7},
      ddc          = {670},
      cid          = {I:(DE-Juel1)VDB787},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK414},
      shelfmark    = {Chemistry, Multidisciplinary / Chemistry, Physical /
                      Materials Science, Multidisciplinary},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:17279644},
      UT           = {WOS:000243990200015},
      doi          = {10.1021/la062184m},
      url          = {https://juser.fz-juelich.de/record/56003},
}