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@ARTICLE{Li:56407,
author = {Li, H.-F. and Su, Y. and Persson, J. and Meuffels, P. and
Walter, J. M. and Skowronek, R. and Brückel, T.},
title = {{N}eutron-diffraction study of structural transition and
magnetic order in orthorhombic and rhombohedral
{L}a7/8{S}r1/8{M}n1-gamma{O}3+delta},
journal = {Journal of physics / Condensed matter},
volume = {19},
issn = {0953-8984},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {PreJuSER-56407},
pages = {176226-1 -176226-12},
year = {2007},
note = {Record converted from VDB: 12.11.2012},
abstract = {We report on a systematic neutron powder diffraction (NPD)
study of polycrystalline La(7/8)Sr(1/8)Mn(1-γ)O(3+δ)
compounds. We investigated the structural and magnetic
phases and transitions in the temperature range between 10
and 900 K for two different samples: an Ar-annealed sample
with an orthorhombic Pbnm (Z = 4; O) structure at room
temperature and an air-sintered sample with a rhombohedral
[Formula: see text] (Z = 2;R) structure at room temperature.
At higher temperatures, above 400 K, both samples exhibit a
rhombohedral structure. For the Ar-annealed sample, a
Jahn-Teller (JT) transition occurs in the orthorhombic phase
at about 298 K with very large variations in the Mn-O2' and
Mn-O2 bond lengths and Mn-O1-Mn bond angle on cooling from
298 to 180 K. For this sample the ferromagnetic moment at
10 K in the magnetic space group Pb'n'm amounts to
3.22(5) μ(B)/Mn. In contrast, the air-sintered sample
undergoes on cooling a structural transition from
rhombohedral (R) to orthorhombic (O) with a mixed phase of
nearly equal R and O repartition at 120 K. Ferromagnetic
order develops in this sample at about 240 K with a
low-temperature moment of 3.35(4) μ(B)/Mn at 10 K. The
coherent JT distortion in its orthorhombic phase occurs
below some 170 K. In addition, we have determined the
coherent JT distortion parameter Δ, the tolerance factor t
and the one-electron bandwidth W of the e(g)-band.},
keywords = {J (WoSType)},
cin = {IFF-4 / IFF-5 / Jülich Centre for Neutron Science JCNS
(JCNS) ; JCNS / IFF-6 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)VDB784 / I:(DE-Juel1)VDB785 /
I:(DE-Juel1)JCNS-20121112 / I:(DE-Juel1)VDB786 /
$I:(DE-82)080009_20140620$},
pnm = {Kondensierte Materie / Großgeräte für die Forschung mit
Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK414 / G:(DE-Juel1)FUEK415},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:21690971},
UT = {WOS:000246556400038},
doi = {10.1088/0953-8984/19/17/176226},
url = {https://juser.fz-juelich.de/record/56407},
}