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000056505 084__ $$2WoS$$aChemistry, Physical
000056505 084__ $$2WoS$$aNanoscience & Nanotechnology
000056505 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000056505 1001_ $$0P:(DE-Juel1)VDB34540$$aLüssem, B.$$b0$$uFZJ
000056505 245__ $$aElectrical Characterization of Biphenylalkanethiol SAMs
000056505 260__ $$aWashington, DC$$bSoc.$$c2007
000056505 300__ $$a6392
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000056505 440_0 $$016841$$aJournal of Physical Chemistry C$$v111$$x1932-7447
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000056505 520__ $$aThe electron-transfer properties of a full-coverage self-assembled monolayer of biphenylethanethiol (CH3-C6H4-C6H4-(CH2)(2)-SH, BP2) is studied by current versus distance spectroscopy. With this, the electrical properties of different functional groups in one molecule are vertically resolved. The current versus distance plot is shown to consist of three different parts, whose logarithmic slope is interpreted as the decay length of the vacuum, the biphenyl group, and the alkane chain. This finding is described in a trilayer tunnel junction model and the decay constant, beta(Ph), of the tunneling current through the biphenyl group is estimated. Besides characterizing the biphenylalkanethiol monolayers electrically, the structure of these layers is determined by UHV-STM. Two new structures with rectangular (4 x 6 root 3) lattices are identified for 4'-methyl-1,1'-biphenyl-4-ethanethiol self-assembled monolayers on (111)-oriented gold surfaces.
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000056505 7001_ $$0P:(DE-Juel1)VDB42769$$aMüller-Meskamp, L.$$b1$$uFZJ
000056505 7001_ $$0P:(DE-Juel1)130751$$aKarthäuser, S.$$b2$$uFZJ
000056505 7001_ $$0P:(DE-HGF)0$$aHomberger, M.$$b3
000056505 7001_ $$0P:(DE-HGF)0$$aSimon, U.$$b4
000056505 7001_ $$0P:(DE-Juel1)131022$$aWaser, R.$$b5$$uFZJ
000056505 773__ $$0PERI:(DE-600)2256522-X$$a10.1021/jp067459l$$gVol. 111, p. 6392$$p6392$$q111<6392$$tThe @journal of physical chemistry <Washington, DC> / C$$v111$$x1932-7447$$y2007
000056505 8567_ $$uhttp://dx.doi.org/10.1021/jp067459l
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000056505 9201_ $$0I:(DE-Juel1)VDB786$$d31.12.2010$$gIFF$$kIFF-6$$lElektronische Materialien$$x0
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