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000056664 084__ $$2WoS$$aPhysics, Condensed Matter
000056664 1001_ $$0P:(DE-Juel1)VDB37196$$aLounis, S.$$b0$$uFZJ
000056664 245__ $$aNoncollinear magnetism of Cr and Mn nanoclusters on Ni(111): Changing the magnetic configuration atom by atom
000056664 260__ $$aCollege Park, Md.$$bAPS$$c2007
000056664 300__ $$a174436
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000056664 520__ $$aThe Korringa-Kohn-Rostoker Green-function method for noncollinear magnetic structures was applied on Mn and Cr nanoclusters deposited on the Ni(111) surface. We consider various dimers, trimers, and tetramers. We obtain collinear and noncollinear magnetic solutions, brought about by the competition of antiferromagnetic interactions. It is found that the triangular geometry of the Ni(111) substrate, together with the intracluster antiferromagnetic interactions, is the main cause of the noncollinear states, which are secondarily affected by the cluster-substrate exchange interactions. The stabilization energy of the noncollinear, compared to the collinear, states is calculated to be typically of the order of 100 meV/atom, while multiple local-energy minima are found, corresponding to different noncollinear states, differing typically by 1-10 meV/atom. Open structures exhibit sizable total moments, while compact clusters tend to have very small total moments, resulting from the complex frustration mechanisms in these systems.
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000056664 7001_ $$0P:(DE-Juel1)130823$$aMavropoulos, Ph.$$b1$$uFZJ
000056664 7001_ $$0P:(DE-Juel1)131057$$aZeller, R.$$b2$$uFZJ
000056664 7001_ $$0P:(DE-Juel1)130612$$aDederichs, P. H.$$b3$$uFZJ
000056664 7001_ $$0P:(DE-Juel1)130548$$aBlügel, S.$$b4$$uFZJ
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000056664 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevB.75.174436
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