000057129 001__ 57129
000057129 005__ 20200402210345.0
000057129 0247_ $$2pmid$$apmid:16898857
000057129 0247_ $$2DOI$$a10.1562/2006-07-14-RC-969
000057129 0247_ $$2WOS$$aWOS:000241426600032
000057129 037__ $$aPreJuSER-57129
000057129 041__ $$aeng
000057129 082__ $$a570
000057129 084__ $$2WoS$$aBiochemistry & Molecular Biology
000057129 084__ $$2WoS$$aBiophysics
000057129 1001_ $$0P:(DE-HGF)0$$aBadura, A.$$b0
000057129 245__ $$aLight-driven water splitting for (bio-)hydrogen production: photosystem 2 as the central part of a bioelectrochemical device
000057129 260__ $$aMalden, Mass.$$bWiley-Blackwell$$c2006
000057129 300__ $$a1385 - 1390
000057129 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
000057129 3367_ $$2DataCite$$aOutput Types/Journal article
000057129 3367_ $$00$$2EndNote$$aJournal Article
000057129 3367_ $$2BibTeX$$aARTICLE
000057129 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000057129 3367_ $$2DRIVER$$aarticle
000057129 440_0 $$015281$$aPhotochemistry and Photobiology$$v82$$x0031-8655$$y5
000057129 500__ $$aRecord converted from VDB: 12.11.2012
000057129 520__ $$aTo establish a semiartificial device for (bio-)hydrogen production utilizing photosynthetic water oxidation, we report on the immobilization of a Photosystem 2 on electrode surfaces. For this purpose, an isolated Photosystem 2 with a genetically introduced His tag from the cyanobacterium Thermosynechococcus elongatus was attached onto gold electrodes modified with thiolates bearing terminal Ni(II)-nitrilotriacetic acid groups. Surface enhanced infrared absorption spectroscopy showed the binding kinetics of Photosystem 2, whereas surface plasmon resonance measurements allowed the amount of protein adsorbed to be quantified. On the basis of these data, the surface coverage was calculated to be 0.29 pmol protein cm(-2), which is in agreement with the formation of a monomolecular film on the electrode surface. Upon illumination, the generation of a photocurrent was observed with current densities of up to 14 microA cm(-2) . This photocurrent is clearly dependent on light quality showing an action spectrum similar to an isolated Photosystem 2. The achieved current densities are equivalent to the highest reported oxygen evolution activities in solution under comparable conditions.
000057129 536__ $$0G:(DE-Juel1)FUEK409$$2G:(DE-HGF)$$aFunktion und Dysfunktion des Nervensystems$$cP33$$x0
000057129 588__ $$aDataset connected to Web of Science, Pubmed
000057129 650_2 $$2MeSH$$aElectrochemistry: methods
000057129 650_2 $$2MeSH$$aElectrodes
000057129 650_2 $$2MeSH$$aHydrogen: metabolism
000057129 650_2 $$2MeSH$$aKinetics
000057129 650_2 $$2MeSH$$aLight
000057129 650_2 $$2MeSH$$aPhotochemistry
000057129 650_2 $$2MeSH$$aPhotosystem II Protein Complex: metabolism
000057129 650_2 $$2MeSH$$aPhotosystem II Protein Complex: radiation effects
000057129 650_2 $$2MeSH$$aSynechococcus: metabolism
000057129 650_2 $$2MeSH$$aSynechococcus: radiation effects
000057129 650_2 $$2MeSH$$aWater: metabolism
000057129 650_7 $$00$$2NLM Chemicals$$aPhotosystem II Protein Complex
000057129 650_7 $$01333-74-0$$2NLM Chemicals$$aHydrogen
000057129 650_7 $$07732-18-5$$2NLM Chemicals$$aWater
000057129 650_7 $$2WoSType$$aJ
000057129 7001_ $$0P:(DE-HGF)0$$aEsper, B.$$b1
000057129 7001_ $$0P:(DE-Juel1)VDB5396$$aAtaka, K.$$b2$$uFZJ
000057129 7001_ $$0P:(DE-HGF)0$$aGrunwald, A.$$b3
000057129 7001_ $$0P:(DE-HGF)0$$aWöll, C.$$b4
000057129 7001_ $$0P:(DE-HGF)0$$aKuhlmann, J.$$b5
000057129 7001_ $$0P:(DE-Juel1)VDB572$$aHeberle, J.$$b6$$uFZJ
000057129 7001_ $$0P:(DE-HGF)0$$aRögner, M.$$b7
000057129 773__ $$0PERI:(DE-600)2048860-9$$a10.1562/2006-07-14-RC-969$$gVol. 82, p. 1385 - 1390$$p1385 - 1390$$q82<1385 - 1390$$tPhotochemistry and photobiology$$v82$$x0031-8655$$y2006
000057129 8567_ $$uhttp://dx.doi.org/10.1562/2006-07-14-RC-969
000057129 909CO $$ooai:juser.fz-juelich.de:57129$$pVDB
000057129 9131_ $$0G:(DE-Juel1)FUEK409$$bGesundheit$$kP33$$lFunktion und Dysfunktion des Nervensystems$$vFunktion und Dysfunktion des Nervensystems$$x0
000057129 9141_ $$aNachtrag$$y2006
000057129 915__ $$0StatID:(DE-HGF)0010$$aJCR/ISI refereed
000057129 9201_ $$0I:(DE-Juel1)VDB58$$d31.12.2006$$gIBI$$kIBI-2$$lBiologische Strukturforschung$$x1
000057129 970__ $$aVDB:(DE-Juel1)89874
000057129 980__ $$aVDB
000057129 980__ $$aConvertedRecord
000057129 980__ $$ajournal
000057129 980__ $$aI:(DE-Juel1)ISB-2-20090406
000057129 980__ $$aUNRESTRICTED
000057129 980__ $$aI:(DE-Juel1)ICS-6-20110106
000057129 981__ $$aI:(DE-Juel1)IBI-7-20200312
000057129 981__ $$aI:(DE-Juel1)ISB-2-20090406
000057129 981__ $$aI:(DE-Juel1)ICS-6-20110106