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@ARTICLE{GroudevaZotova:57170,
author = {Groudeva-Zotova, S. and Kozhuharova, R. and Elefant, D. and
Mühl, T. and Schneider, C. M. and Mönch, I.},
title = {{P}hase composition and magnetic characteristics of
{F}e-filled multi-walled carbon nanotubes},
journal = {Journal of magnetism and magnetic materials},
volume = {306},
issn = {0304-8853},
address = {Amsterdam},
publisher = {North-Holland Publ. Co.},
reportid = {PreJuSER-57170},
pages = {40 - 50},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {The work addresses the correlation between the phase
composition and the magnetic characteristics of aligned
Fe-filled multi-walled carbon nanotubes (Fe-MWCNTs) grown by
pyrolysis of ferrocene on oxidized Si substrates. In a
combinatorial approach we exploited the extremely high
gradients of the technological parameters temperature and
ferrocene flow across the surface of a substrate positioned
close to the reactor wall to obtain a large variation in the
structural and magnetic properties of the Fe-MWCNTs. In this
way, we established several clear correlations between the
Fe-filling phase composition and the overall magnetic
characteristics of the aligned Fe-MWCNTs. The alpha-Fe rich
samples, which possess a more ordered graphitic sheet
structure, a higher degree of preferred crystalline
orientation of the metal filling and much larger metal
crystallites in comparison with the carbide-rich samples,
show a much stronger magnetic anisotropy with easy axis
perpendicular to the substrate and unusually high values of
the coercive field H-c and the saturation field H-s. The
changes in the measured saturation magnetisation M-s and the
H-c values correlate well with the variation of the alpha-Fe
content and the filling crystallinity. A special annealing
treatment of the samples causes a distinct increase of the
alpha-Fe quantity and an increase of the measured average
grain size. The respective magnetic characteristics show a
significant increase of the overall magnetic moment and
decrease of the coercive field. The correlation between the
structural and the magnetic characteristics of the annealed
samples matches quite well the respective correlations in
the case of as-deposited samples. (C) 2006 Elsevier B.V. All
rights reserved.},
keywords = {J (WoSType)},
cin = {IFF-IEE / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)VDB38 / $I:(DE-82)080009_20140620$},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK414},
shelfmark = {Materials Science, Multidisciplinary / Physics, Condensed
Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000240760800007},
doi = {10.1016/j.jmmm.2006.02.103},
url = {https://juser.fz-juelich.de/record/57170},
}