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@ARTICLE{Krmer:57394,
author = {Krämer, M. and Schiller, C. and Voigt, Ch. and Schlager,
H. and Popp, P. J.},
title = {{A} climatological view of {HNO}3 partitioning in cirrus
clouds},
journal = {Quarterly journal of the Royal Meteorological Society},
volume = {134},
issn = {0035-9009},
address = {Weinheim [u.a.]},
publisher = {Wiley},
reportid = {PreJuSER-57394},
pages = {905 - 912},
year = {2008},
note = {The authors thank the coordinators and all teams
contributing to the field experiments compiled in the study
presented here. Progress in the challenging task of
providing an estimate of the nitric acid content of ice for
most atmospheric conditions is only possible due to the
large effort flowing into all the experiments.Funding from
various agencies for the different projects is acknowledged,
in particular for SCOUT-O3 which is funded by the EC within
FP6 under contract GOCE-CT-2004-505390. C. Voigt appreciates
funding by the Helmholtz Young Investigators Fund and the
SFB-641 TROP-ICE. The authors also would like to thank Bernd
Kaarcher for stimulating discussions. As always, Rolf P.
Muller is gratefully acknowledged.},
abstract = {A new in situ climatology of cirrus ice water content (IWC)
is used, together with observed molar ratios of HNO3/H2O in
cirrus ice particles, to estimate the range of HNO3 content
in cirrus ice in the temperature interval 185-240 K. We find
that nearly over the complete temperature range HNO3
percentages in ice between 0.01 and $100\%$ are possible in
cirrus clouds and that IWC is a major parameter determining
the content of HNO3 in ice at given temperatures.
Considering average conditions, the HNO3 content increases
with decreasing temperature from $1\%$ to about $10\%$ in
the range 240-200 K. For colder ice clouds, the average HNO3
content again decreases down to $6\%.$ At higher
temperatures, less efficient HNO3 uptake limits the HNO3
content in cirrus ice, while at low temperatures small IWCs
permit only little HNO3 in ice, thus causing the
convex-shaped average HNO3 content curve. The highest HNO3
content is expected in tropical ice clouds with very large
IWCs, especially at temperatures between 190 and 210 K.
Thus, tropical cirrus clouds show the highest potential to
vertically redistribute HNO3. Copyright (C) 2008 Royal
Meteorological Society.},
keywords = {J (WoSType)},
cin = {ICG-1},
ddc = {550},
cid = {I:(DE-Juel1)VDB790},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000259292700008},
doi = {10.1002/qj.253},
url = {https://juser.fz-juelich.de/record/57394},
}