TY - JOUR
AU - Ishida, H.
AU - Wortmann, D.
AU - Liebsch, A.
TI - Electronic structure of SrVO3(001) surfaces: a local-density approximation plus dynamical mean-field theory calculation
JO - Physical review / B
VL - 73
IS - 24
SN - 1098-0121
CY - College Park, Md.
PB - APS
M1 - PreJuSER-57446
SP - 245421
PY - 2006
N1 - Record converted from VDB: 12.11.2012
AB - The influence of local Coulomb correlations on the surface electronic structure of SrVO3, a strongly-correlated metal in a perovskite structure, is investigated for both the SrO-layer and VO2-layer-terminated (001) surfaces. The electronic structure within the local density approximation of a semi-infinite surface is determined using the embedded Green-function approach, and the resultant density of states projected on the V t2g orbitals is used as an input to a subsequent many-body calculation within the dynamical mean field theory (DMFT) and the multiorbital quantum Monte Carlo technique. Qualitatively, the present study confirms the conclusion of recent photoemission experiments and tight-binding DMFT calculations which both indicate that the electronic structure at the surface is more strongly correlated than in the bulk. On a quantitative level significant differences are obtained as a function of orbital polarization at the surface, surface layer relaxation, and SrO vs VO2 surface termination.
KW - J (WoSType)
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000238696900119
DO - DOI:10.1103/PhysRevB.73.245421
UR - https://juser.fz-juelich.de/record/57446
ER -