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000057544 084__ $$2WoS$$aEnvironmental Sciences
000057544 084__ $$2WoS$$aMeteorology & Atmospheric Sciences
000057544 1001_ $$0P:(DE-Juel1)16311$$aPoppe, D.$$b0$$uFZJ
000057544 245__ $$aOH-initiated degradation of several hydrocarbons in the atmosphere simulation chamber SAPHIR
000057544 260__ $$aDordrecht [u.a.]$$bSpringer Science + Business Media B.V$$c2007
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000057544 440_0 $$03073$$aJournal of Atmospheric Chemistry$$v57$$x0167-7764
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000057544 520__ $$aDegradation of isoprene, m-xylene, n-octane, propene, and methacrolein by hydroxyl radicals has been studied in the simulation chamber SAPHIR under burden of trace gases as they are typical for the moderately polluted planetary boundary layer. Measured time series of the hydrocarbon mixing ratios and the OH concentrations were used to determine the rate constants. The hydrocarbons were measured with gas chromatography and proton transfer reaction mass spectrometry. OH was measured with the Julich DOAS (differential optical absorption spectroscopy) instrument. In all cases except methacrolein good agreement was found with the reference rate constants taken from theMaster Chemical Mechanism ( MCM3.1). The data for methacrolein are consistent with the results of Karl et al. ( J. Atmos. Chem 55, 2006, doi:10.1007/s10874-006-9034-x) who reported a 12% smaller value. The degradation of hydrocarbons provides an independent method to analyse precision and accuracy of the OH measurements. A precision of better than 4% over a period of nearly 4 months was found. The accuracy is within the limitations given by the light absorption cross section of OH. Both results are consistent with earlier results by Hausmann et al.
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000057544 65320 $$2Author$$aatmospheric degradation of hydrocarbons
000057544 65320 $$2Author$$ahydroxyl radicals
000057544 65320 $$2Author$$atropospheric ozone
000057544 65320 $$2Author$$an-octane
000057544 65320 $$2Author$$apropene
000057544 65320 $$2Author$$am-xylene
000057544 65320 $$2Author$$aisoprene
000057544 65320 $$2Author$$amethacrolein
000057544 65320 $$2Author$$asimulation chamber
000057544 65320 $$2Author$$ameasurement of atmospheric OH concentrations
000057544 7001_ $$0P:(DE-Juel1)16306$$aBrauers, T.$$b1$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)16317$$aDorn, H.-P.$$b2$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)VDB13401$$aKarl, M.$$b3$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)16346$$aMentel, T.$$b4$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)VDB26256$$aSchlosser, E.$$b5$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)5344$$aTillmann, R.$$b6$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)2367$$aWegener, R.$$b7$$uFZJ
000057544 7001_ $$0P:(DE-Juel1)16324$$aWahner, A.$$b8$$uFZJ
000057544 773__ $$0PERI:(DE-600)1475524-5$$a10.1007/s10874-007-9065-y$$gVol. 57, p. 203 - 214$$p203 - 214$$q57<203 - 214$$tJournal of atmospheric chemistry$$v57$$x0167-7764$$y2007
000057544 8567_ $$uhttp://dx.doi.org/10.1007/s10874-007-9065-y
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