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000057623 017__ $$aCopyright APS. This version is available at http://link.aps.org/abstract/PRE/v74/e031201
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000057623 084__ $$2WoS$$aPhysics, Mathematical
000057623 1001_ $$0P:(DE-Juel1)VDB39943$$aMcPhie, M. G.$$b0$$uFZJ
000057623 245__ $$aViscosity of a binary mixture: Approach to the hydrodynamic limit
000057623 260__ $$aCollege Park, Md.$$bAPS$$c2006
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000057623 520__ $$aWe have used equilibrium and nonequilibrium molecular dynamics simulations to study the solute self-diffusion coefficient and the shear rate dependence of the solution viscosity in solutions of model nanocolloidal particles that range in mass ratio from mu=1 up to mu=50 and size ratio from s=1 up to s=4.03 at various concentrations. The zero shear rate viscosities and the initial rates of shear thinning were determined from data in the shear rate region in which the suspension is strongly shear thinning while the solvent remains Newtonian or is weakly shear thinning. The rate of shear thinning increased dramatically with solute volume fraction, regardless of whether the increase was due to increasing solute size or increasing the solute concentration. In a series of simulations in which the mass ratio was varied while keeping the size ratio fixed at s=1, we found that the approach of the viscosities and self-diffusion coefficients to their limiting mass ratio independent values was well described by a rather simple exponential dependence on mass ratio. The concentration dependence of the limiting infinite mass ratio values of the self-diffusion coefficients and zero shear rate viscosities were determined, and used to compute the hydrodynamic radius R-H of the solute particles by various methods. The values of R-H that were obtained by the different methods were reasonably consistent with each other, and indicated that the radius at which the slip boundary condition holds is slightly smaller than the cross-interaction radius between the solute and solvent particles.
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000057623 7001_ $$0P:(DE-HGF)0$$aDaivis, P. J.$$b1
000057623 7001_ $$0P:(DE-HGF)0$$aSnook, I.K.$$b2
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000057623 8567_ $$uhttp://hdl.handle.net/2128/3028$$uhttp://dx.doi.org/10.1103/PhysRevE.74.031201
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000057623 999C5 $$1J.-P. Hansen$$2Crossref$$oJ.-P. Hansen Theory of Simple Liquids 1986$$tTheory of Simple Liquids$$y1986
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1675379
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.473316
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.58.5845
000057623 999C5 $$1F. Ould-Kaddour$$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.63.011205$$p011205 -$$tPhys. Rev. E$$v63$$y2001
000057623 999C5 $$1I. K. Snook$$2Crossref$$9-- missing cx lookup --$$a10.1016/S0167-7322(02)00158-7$$p405 -$$tJ. Mol. Liq.$$v103-104$$y2003
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1610442
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1017/S0022112083001275
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1017/S0022112083002566
000057623 999C5 $$1A. Einstein$$2Crossref$$oA. Einstein Investigations on the Theory of the Brownian Movement 1956$$tInvestigations on the Theory of the Brownian Movement$$y1956
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1007/BF02188674
000057623 999C5 $$1T. Kihara$$2Crossref$$oT. Kihara Intermolecular Forces 1976$$tIntermolecular Forces$$y1976
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1674820
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/S0378-4371(97)00612-2
000057623 999C5 $$1D. J. Evans$$2Crossref$$oD. J. Evans Statistical Mechanics of Nonequilibrium Liquids 1990$$tStatistical Mechanics of Nonequilibrium Liquids$$y1990
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00268979300100371
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0022-3719/5/15/006
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/0375-9601(92)90335-J
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.467468
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.469006
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000057623 999C5 $$1M. P. Allen$$2Crossref$$oM. P. Allen Computer Simulation of Liquids 1987$$tComputer Simulation of Liquids$$y1987
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.442716
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.473273
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.479358
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/0167-7977(84)90001-7
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000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1678535
000057623 999C5 $$1T. Yamada$$2Crossref$$oT. Yamada 1973$$y1973
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00268978900102421
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/002689798167115
000057623 999C5 $$1G. Marcelli$$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.63.021204$$p021204 -$$tPhys. Rev. E$$v63$$y2002
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00268970210137275
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/S0378-4371(97)00682-1
000057623 999C5 $$1R. I. Tanner$$2Crossref$$oR. I. Tanner Engineering Rheology 2000$$tEngineering Rheology$$y2000
000057623 999C5 $$1R. G. Larson$$2Crossref$$oR. G. Larson The Structure and Rheology of Complex Fluids, Topics in Complex Engineering 1999$$tThe Structure and Rheology of Complex Fluids, Topics in Complex Engineering$$y1999
000057623 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1017/S0022112077001062
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