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@ARTICLE{McPhie:57623,
      author       = {McPhie, M. G. and Daivis, P. J. and Snook, I.K.},
      title        = {{V}iscosity of a binary mixture: {A}pproach to the
                      hydrodynamic limit},
      journal      = {Physical review / E},
      volume       = {74},
      number       = {3},
      issn         = {1539-3755},
      address      = {College Park, Md.},
      publisher    = {APS},
      reportid     = {PreJuSER-57623},
      pages        = {031201},
      year         = {2006},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {We have used equilibrium and nonequilibrium molecular
                      dynamics simulations to study the solute self-diffusion
                      coefficient and the shear rate dependence of the solution
                      viscosity in solutions of model nanocolloidal particles that
                      range in mass ratio from mu=1 up to mu=50 and size ratio
                      from s=1 up to s=4.03 at various concentrations. The zero
                      shear rate viscosities and the initial rates of shear
                      thinning were determined from data in the shear rate region
                      in which the suspension is strongly shear thinning while the
                      solvent remains Newtonian or is weakly shear thinning. The
                      rate of shear thinning increased dramatically with solute
                      volume fraction, regardless of whether the increase was due
                      to increasing solute size or increasing the solute
                      concentration. In a series of simulations in which the mass
                      ratio was varied while keeping the size ratio fixed at s=1,
                      we found that the approach of the viscosities and
                      self-diffusion coefficients to their limiting mass ratio
                      independent values was well described by a rather simple
                      exponential dependence on mass ratio. The concentration
                      dependence of the limiting infinite mass ratio values of the
                      self-diffusion coefficients and zero shear rate viscosities
                      were determined, and used to compute the hydrodynamic radius
                      R-H of the solute particles by various methods. The values
                      of R-H that were obtained by the different methods were
                      reasonably consistent with each other, and indicated that
                      the radius at which the slip boundary condition holds is
                      slightly smaller than the cross-interaction radius between
                      the solute and solvent particles.},
      keywords     = {J (WoSType)},
      cin          = {IFF-IWM},
      ddc          = {530},
      cid          = {I:(DE-Juel1)VDB343},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK414},
      shelfmark    = {Physics, Fluids $\&$ Plasmas / Physics, Mathematical},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000240870100037},
      doi          = {10.1103/PhysRevE.74.031201},
      url          = {https://juser.fz-juelich.de/record/57623},
}