001     57623
005     20240619083429.0
017 _ _ |a Copyright APS. This version is available at http://link.aps.org/abstract/PRE/v74/e031201
024 7 _ |a 10.1103/PhysRevE.74.031201
|2 DOI
024 7 _ |a WOS:000240870100037
|2 WOS
024 7 _ |a 2128/3028
|2 Handle
037 _ _ |a PreJuSER-57623
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Physics, Fluids & Plasmas
084 _ _ |2 WoS
|a Physics, Mathematical
100 1 _ |a McPhie, M. G.
|b 0
|u FZJ
|0 P:(DE-Juel1)VDB39943
245 _ _ |a Viscosity of a binary mixture: Approach to the hydrodynamic limit
260 _ _ |a College Park, Md.
|b APS
|c 2006
264 _ 1 |3 online
|2 Crossref
|b American Physical Society (APS)
|c 2006-09-06
264 _ 1 |3 print
|2 Crossref
|b American Physical Society (APS)
|c 2006-09-01
300 _ _ |a 031201
336 7 _ |a Journal Article
|0 PUB:(DE-HGF)16
|2 PUB:(DE-HGF)
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
|0 0
|2 EndNote
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a article
|2 DRIVER
440 _ 0 |a Physical Review E
|x 1539-3755
|0 4924
|v 74
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a We have used equilibrium and nonequilibrium molecular dynamics simulations to study the solute self-diffusion coefficient and the shear rate dependence of the solution viscosity in solutions of model nanocolloidal particles that range in mass ratio from mu=1 up to mu=50 and size ratio from s=1 up to s=4.03 at various concentrations. The zero shear rate viscosities and the initial rates of shear thinning were determined from data in the shear rate region in which the suspension is strongly shear thinning while the solvent remains Newtonian or is weakly shear thinning. The rate of shear thinning increased dramatically with solute volume fraction, regardless of whether the increase was due to increasing solute size or increasing the solute concentration. In a series of simulations in which the mass ratio was varied while keeping the size ratio fixed at s=1, we found that the approach of the viscosities and self-diffusion coefficients to their limiting mass ratio independent values was well described by a rather simple exponential dependence on mass ratio. The concentration dependence of the limiting infinite mass ratio values of the self-diffusion coefficients and zero shear rate viscosities were determined, and used to compute the hydrodynamic radius R-H of the solute particles by various methods. The values of R-H that were obtained by the different methods were reasonably consistent with each other, and indicated that the radius at which the slip boundary condition holds is slightly smaller than the cross-interaction radius between the solute and solvent particles.
536 _ _ |a Kondensierte Materie
|c P54
|2 G:(DE-HGF)
|0 G:(DE-Juel1)FUEK414
|x 0
542 _ _ |i 2006-09-06
|2 Crossref
|u http://link.aps.org/licenses/aps-default-license
588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
|2 WoSType
700 1 _ |a Daivis, P. J.
|b 1
|0 P:(DE-HGF)0
700 1 _ |a Snook, I.K.
|b 2
|0 P:(DE-HGF)0
773 1 8 |a 10.1103/physreve.74.031201
|b American Physical Society (APS)
|d 2006-09-06
|n 3
|p 031201
|3 journal-article
|2 Crossref
|t Physical Review E
|v 74
|y 2006
|x 1539-3755
773 _ _ |a 10.1103/PhysRevE.74.031201
|g Vol. 74, p. 031201
|p 031201
|n 3
|q 74<031201
|0 PERI:(DE-600)2844562-4
|t Physical review / E
|v 74
|y 2006
|x 1539-3755
856 7 _ |u http://dx.doi.org/10.1103/PhysRevE.74.031201
|u http://hdl.handle.net/2128/3028
856 4 _ |u https://juser.fz-juelich.de/record/57623/files/BinaryViscosity_Submission.pdf
|y OpenAccess
856 4 _ |u https://juser.fz-juelich.de/record/57623/files/BinaryViscosity_Submission.jpg?subformat=icon-1440
|x icon-1440
|y OpenAccess
856 4 _ |u https://juser.fz-juelich.de/record/57623/files/BinaryViscosity_Submission.jpg?subformat=icon-180
|x icon-180
|y OpenAccess
856 4 _ |u https://juser.fz-juelich.de/record/57623/files/BinaryViscosity_Submission.jpg?subformat=icon-640
|x icon-640
|y OpenAccess
909 C O |o oai:juser.fz-juelich.de:57623
|p openaire
|p open_access
|p driver
|p VDB
|p dnbdelivery
913 1 _ |k P54
|v Kondensierte Materie
|l Kondensierte Materie
|b Materie
|z entfällt bis 2009
|0 G:(DE-Juel1)FUEK414
|x 0
914 1 _ |a Nachtrag
|y 2006
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
915 _ _ |2 StatID
|0 StatID:(DE-HGF)0510
|a OpenAccess
920 1 _ |k IFF-IWM
|l Weiche Materie
|d 31.12.2006
|g IFF
|0 I:(DE-Juel1)VDB343
|x 0
970 _ _ |a VDB:(DE-Juel1)90647
980 1 _ |a FullTexts
980 _ _ |a VDB
980 _ _ |a JUWEL
980 _ _ |a ConvertedRecord
980 _ _ |a journal
980 _ _ |a I:(DE-Juel1)ICS-3-20110106
980 _ _ |a UNRESTRICTED
980 _ _ |a FullTexts
981 _ _ |a I:(DE-Juel1)ICS-3-20110106
999 C 5 |1 J.-P. Hansen
|y 1986
|2 Crossref
|t Theory of Simple Liquids
|o J.-P. Hansen Theory of Simple Liquids 1986
999 C 5 |a 10.1063/1.1675379
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.473316
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1103/PhysRevE.58.5845
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1103/PhysRevE.63.011205
|9 -- missing cx lookup --
|1 F. Ould-Kaddour
|p 011205 -
|2 Crossref
|t Phys. Rev. E
|v 63
|y 2001
999 C 5 |a 10.1016/S0167-7322(02)00158-7
|9 -- missing cx lookup --
|1 I. K. Snook
|p 405 -
|2 Crossref
|t J. Mol. Liq.
|v 103-104
|y 2003
999 C 5 |a 10.1063/1.1610442
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1017/S0022112083001275
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1017/S0022112083002566
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 A. Einstein
|y 1956
|2 Crossref
|t Investigations on the Theory of the Brownian Movement
|o A. Einstein Investigations on the Theory of the Brownian Movement 1956
999 C 5 |a 10.1007/BF02188674
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 T. Kihara
|y 1976
|2 Crossref
|t Intermolecular Forces
|o T. Kihara Intermolecular Forces 1976
999 C 5 |a 10.1063/1.1674820
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/S0378-4371(97)00612-2
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 D. J. Evans
|y 1990
|2 Crossref
|t Statistical Mechanics of Nonequilibrium Liquids
|o D. J. Evans Statistical Mechanics of Nonequilibrium Liquids 1990
999 C 5 |a 10.1080/00268979300100371
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1088/0022-3719/5/15/006
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/0375-9601(92)90335-J
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.467468
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.469006
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/S0378-4371(97)00134-9
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/S0378-4754(97)00091-8
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 M. P. Allen
|y 1987
|2 Crossref
|t Computer Simulation of Liquids
|o M. P. Allen Computer Simulation of Liquids 1987
999 C 5 |a 10.1063/1.442716
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.473273
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.479358
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/0167-7977(84)90001-7
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.1675378
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1063/1.1678535
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 T. Yamada
|y 1973
|2 Crossref
|o T. Yamada 1973
999 C 5 |a 10.1080/00268978900102421
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1080/002689798167115
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1103/PhysRevE.63.021204
|9 -- missing cx lookup --
|1 G. Marcelli
|p 021204 -
|2 Crossref
|t Phys. Rev. E
|v 63
|y 2002
999 C 5 |a 10.1080/00268970210137275
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/S0378-4371(97)00682-1
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |1 R. I. Tanner
|y 2000
|2 Crossref
|t Engineering Rheology
|o R. I. Tanner Engineering Rheology 2000
999 C 5 |1 R. G. Larson
|y 1999
|2 Crossref
|t The Structure and Rheology of Complex Fluids, Topics in Complex Engineering
|o R. G. Larson The Structure and Rheology of Complex Fluids, Topics in Complex Engineering 1999
999 C 5 |a 10.1017/S0022112077001062
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1039/dc9837600151
|9 -- missing cx lookup --
|2 Crossref
999 C 5 |a 10.1016/0375-9601(88)90501-4
|9 -- missing cx lookup --
|2 Crossref


LibraryCollectionCLSMajorCLSMinorLanguageAuthor
Marc 21