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@ARTICLE{Wahner:57695,
      author       = {Wahner, A. and Moortgat, G. K.},
      title        = {{D}ie {A}tmosphäre als photochemischer {R}eaktor},
      journal      = {Chemie in unserer Zeit},
      volume       = {41},
      issn         = {0009-2851},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {PreJuSER-57695},
      pages        = {192 - 198},
      year         = {2007},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The troposphere is a very large photochemical reactor,
                      which transforms enormous quantities of trace gases and
                      aerosols. Future increases of anthropogenic and natural
                      emissions and aerosol formation will continue to change the
                      status of the troposphere and the climate. Here the
                      self-cleansing capability of the troposphere plays a
                      decisive role. The tropospheric oxidation is initiated
                      through a series of oxidants, especially, by the hydroxyl
                      radical, OH, but also by ozone, O-3, and the nitrate
                      radical, NO3. By their reaction with trace gas molecules, OH
                      radicals are not consumed, but regenerated in catalytic
                      cycles, where the concentration of nitrogen oxides plays c
                      dominant role. This mechanism is general applicable to
                      simple examples of the photochemical reaction system of the
                      troposphere: most reactions of OH radicals with atmospheric
                      trace gas molecules (e.g. methane, anthropogenic or biogenic
                      emitted organic compounds) lead to chain reactions, which
                      regenerate OH radicals. It clarifies that the degradation of
                      trace gas species in a NO-containing atmosphere is
                      irrevocably connected with the production of ozone. It also
                      shows that the self-cleansing capability and consequently
                      air quality and climate change of the troposphere are
                      crucially influenced by the tropospheric photochemistry and
                      the emissions.},
      keywords     = {J (WoSType)},
      cin          = {ICG-2 / JARA-ENERGY / JARA-SIM},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB791 / $I:(DE-82)080011_20140620$ /
                      I:(DE-Juel1)VDB1045},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK406},
      shelfmark    = {Chemistry, Multidisciplinary},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000247706600005},
      doi          = {10.1002/ciuz.200700429},
      url          = {https://juser.fz-juelich.de/record/57695},
}