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@ARTICLE{Lee:57739,
author = {Lee, H. and Park, J. S. and Kim, H. and Yoon, K. B. and
Seeck, O. H. and Kim, D. H. and Seo, S. H. and Kang, H. C.
and Noh, D. Y.},
title = {{C}haracterization of molecular linkages placed between
zeolite microcrystal monolayers and a substrate with {X}-ray
reflectivity},
journal = {Langmuir},
volume = {22},
issn = {0743-7463},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {PreJuSER-57739},
pages = {2598 - 2604},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {We prepared silicalite-1 microcrystal (MC) monolayers on a
Si wafer using two different types of molecular linkages,
namely, through chloropropyl (CP) groups and through
CP/polyethylene imine/CP groups. Whereas the scanning
electron microscope images of the two MC monolayers look
very much alike but hardly give any information on the
nature of molecular linkage between the monolayers and the
substrate, their reflectivity curves are distinctively
different, despite the fact that the thicknesses of the
molecular linkage layers ( approximately 10-20 A) are
negligibly small compared to the thicknesses of MC
monolayers, ( approximately 3200 A). On the basis of the
atomic force microscopic images of the MC surfaces, a rough
surface layer with the thickness of approximately 160 A was
introduced onto the surface of each MC to conduct a
meaningful simulation of the curves with the recursive
Parratt formalism. The obtained thickness, roughness, and
density of each layer were reasonable, indicating that X-ray
reflectivity is a very useful tool for the characterization
of very thin layers of molecular linkages existing between
much thicker MC monolayers and the substrate.},
keywords = {Microscopy, Electron, Scanning / Spectrophotometry,
Ultraviolet / X-Rays / Zeolites: chemistry / Zeolites (NLM
Chemicals) / J (WoSType)},
cin = {IFF-ISM},
ddc = {670},
cid = {I:(DE-Juel1)VDB342},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK414},
shelfmark = {Chemistry, Multidisciplinary / Chemistry, Physical /
Materials Science, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:16519459},
UT = {WOS:000236009900033},
doi = {10.1021/la051856q},
url = {https://juser.fz-juelich.de/record/57739},
}