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@ARTICLE{Dentener:57797,
author = {Dentener, F. and Drevet, J. and Lamarque, J. F. and Bey, I.
and Eickhout, B. and Fiore, A. M. and Hauglustaine, D. and
Horowitz, L. W. and Krol, M. and Kulshrestha, U.C. and
Lawrence, M. and Galy-Lacaux, C. and Rast, S. and Shindell,
D. and Stevenson, D. and Van Noije, T. and Atherton, C. and
Bell, N. and Bergmann, D. and Butler, T. and Cofala, J. and
Collins, B. and Doherty, R. and Ellingsen, K. and Galloway,
J. and Gauss, M. and Montanaro, V. and Müller, J. F. and
Pitari, G. and Rodriguez, J. and Sanderson, M. and Solmon,
F. and Strahan, S. and Schultz, M. and Sudo, K. and Szopa,
S. and Wild, O.},
title = {{N}itrogen and sulfur deposition on regional and global
scales: {A} multimodel evaluation},
journal = {Global biogeochemical cycles},
volume = {20},
issn = {0886-6236},
address = {Washington, DC},
publisher = {AGU},
reportid = {PreJuSER-57797},
pages = {GB4003},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {[1] We use 23 atmospheric chemistry transport models to
calculate current and future (2030) deposition of reactive
nitrogen (NOy, NHx) and sulfate (SOx) to land and ocean
surfaces. The models are driven by three emission scenarios:
( 1) current air quality legislation (CLE); ( 2) an
optimistic case of the maximum emissions reductions
currently technologically feasible ( MFR); and ( 3) the
contrasting pessimistic IPCC SRES A2 scenario. An extensive
evaluation of the present-day deposition using nearly all
information on wet deposition available worldwide shows a
good agreement with observations in Europe and North
America, where 60 - $70\%$ of the model-calculated wet
deposition rates agree to within +/- $50\%$ with
quality-controlled measurements. Models systematically
overestimate NHx deposition in South Asia, and underestimate
NOy deposition in East Asia. We show that there are
substantial differences among models for the removal
mechanisms of NOy, NHx, and SOx, leading to +/- 1 sigma
variance in total deposition fluxes of about $30\%$ in the
anthropogenic emissions regions, and up to a factor of 2
outside. In all cases the mean model constructed from the
ensemble calculations is among the best when comparing to
measurements. Currently, 36 - $51\%$ of all NOy, NHx, and
SOx is deposited over the ocean, and 50 - $80\%$ of the
fraction of deposition on land falls on natural
(nonagricultural) vegetation. Currently, $11\%$ of the
world's natural vegetation receives nitrogen deposition in
excess of the "critical load'' threshold of 1000 mg(N) m(-2)
yr(-1). The regions most affected are the United States
$(20\%$ of vegetation), western Europe ( $30\%),$ eastern
Europe ( $80\%),$ South Asia $(60\%),$ East Asia $40\%),$
southeast Asia $(30\%),$ and Japan $(50\%).$ Future
deposition fluxes are mainly driven by changes in emissions,
and less importantly by changes in atmospheric chemistry and
climate. The global fraction of vegetation exposed to
nitrogen loads in excess of 1000 mg(N) m(-2) yr(-1)
increases globally to $17\%$ for CLE and $25\%$ for A2. In
MFR, the reductions in NOy are offset by further increases
for NHx deposition. The regions most affected by exceedingly
high nitrogen loads for CLE and A2 are Europe and Asia, but
also parts of Africa.},
keywords = {J (WoSType)},
cin = {ICG-2},
ddc = {550},
cid = {I:(DE-Juel1)VDB791},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Environmental Sciences / Geosciences, Multidisciplinary /
Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000241700200001},
doi = {10.1029/2005GB002672},
url = {https://juser.fz-juelich.de/record/57797},
}