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000059030 084__ $$2WoS$$aPhysics, Condensed Matter
000059030 1001_ $$0P:(DE-HGF)0$$aUeba, H.$$b0
000059030 245__ $$aAction spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope
000059030 260__ $$aCollege Park, Md.$$bAPS$$c2007
000059030 300__ $$a041403
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000059030 520__ $$aWe propose an action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope (STM). Calculations of the inelastic tunneling current for excitation of the C-O stretch mode of the CO molecule on metal surfaces are combined with a theory which describes how the energy in the vibrational mode is transferred to a reaction coordinate mode to overcome the activation barrier. The calculated rate for CO hopping on Pd (110) as a function of the bias voltage agrees with the experimental result. It is proposed that the second derivative of the reaction rate with respect to the bias voltage is related to the vibrational density of states, which usually cannot be directly observed in STM inelastic electron tunneling spectroscopy when a molecule motion is induced by vibrational excitation.
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000059030 7001_ $$0P:(DE-Juel1)130885$$aPersson, B. N. J.$$b1$$uFZJ
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000059030 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevB.75.041403
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