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001     59030
005     20230426083231.0
024 7 _ |2 DOI
|a 10.1103/PhysRevB.75.041403
024 7 _ |2 WOS
|a WOS:000243895600015
037 _ _ |a PreJuSER-59030
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Physics, Condensed Matter
100 1 _ |a Ueba, H.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope
260 _ _ |a College Park, Md.
|b APS
|c 2007
300 _ _ |a 041403
336 7 _ |a Journal Article
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336 7 _ |a Output Types/Journal article
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336 7 _ |a Journal Article
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336 7 _ |a ARTICLE
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336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a article
|2 DRIVER
440 _ 0 |a Physical Review B
|x 1098-0121
|0 4919
|v 75
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a We propose an action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope (STM). Calculations of the inelastic tunneling current for excitation of the C-O stretch mode of the CO molecule on metal surfaces are combined with a theory which describes how the energy in the vibrational mode is transferred to a reaction coordinate mode to overcome the activation barrier. The calculated rate for CO hopping on Pd (110) as a function of the bias voltage agrees with the experimental result. It is proposed that the second derivative of the reaction rate with respect to the bias voltage is related to the vibrational density of states, which usually cannot be directly observed in STM inelastic electron tunneling spectroscopy when a molecule motion is induced by vibrational excitation.
536 _ _ |a Kondensierte Materie
|c P54
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542 _ _ |i 2007-01-05
|2 Crossref
|u http://link.aps.org/licenses/aps-default-license
588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
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700 1 _ |a Persson, B. N. J.
|b 1
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|0 P:(DE-Juel1)130885
773 1 8 |a 10.1103/physrevb.75.041403
|b American Physical Society (APS)
|d 2007-01-05
|n 4
|p 041403
|3 journal-article
|2 Crossref
|t Physical Review B
|v 75
|y 2007
|x 1098-0121
773 _ _ |a 10.1103/PhysRevB.75.041403
|g Vol. 75, p. 041403
|p 041403
|n 4
|q 75<041403
|0 PERI:(DE-600)2844160-6
|t Physical review / B
|v 75
|y 2007
|x 1098-0121
856 7 _ |u http://dx.doi.org/10.1103/PhysRevB.75.041403
856 4 _ |u https://juser.fz-juelich.de/record/59030/files/FZJ-59030.pdf
|y OpenAccess
|z Published final document.
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913 1 _ |k P54
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914 1 _ |y 2007
915 _ _ |0 StatID:(DE-HGF)0010
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915 _ _ |0 LIC:(DE-HGF)APS-112012
|a American Physical Society Transfer of Copyright Ag
|2 HGFVOC
920 1 _ |k IFF-1
|l Quanten-Theorie der Materialien
|d 31.12.2010
|g IFF
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