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000060999 084__ $$2WoS$$aNanoscience & Nanotechnology
000060999 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000060999 084__ $$2WoS$$aPhysics, Applied
000060999 1001_ $$0P:(DE-Juel1)VDB73384$$aTemirov, R.$$b0$$uFZJ
000060999 245__ $$aKondo effect by controlled cleavage of a single-molecule contact
000060999 260__ $$aBristol$$bIOP Publ.$$c2008
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000060999 520__ $$aConductance measurements of a molecular wire, contacted between an epitaxial molecule-metal bond and the tip of a scanning tunnelling microscope, are reported. Controlled retraction of the tip gradually de-hybridizes the molecule from the metal substrate. This tunes the wire into the Kondo regime in which the renormalized molecular transport orbital serves as a spin impurity at half-filling and the Kondo resonance opens up an additional transport channel. Numerical renormalization group simulations suggest this type of behaviour to be generic for a common class of metal-molecule bonds. The results demonstrate a new approach to single-molecule experiments with atomic-scale contact control and prepare the way for the ab initio simulation of many-body transport through single-molecule junctions.
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000060999 7001_ $$0P:(DE-HGF)0$$aLassise, A.$$b1
000060999 7001_ $$0P:(DE-HGF)0$$aAnders, F. B.$$b2
000060999 7001_ $$0P:(DE-Juel1)128791$$aTautz, F. S.$$b3$$uFZJ
000060999 773__ $$0PERI:(DE-600)1362365-5$$a10.1088/0957-4484/19/6/065401$$gVol. 19, p. 065401$$p065401$$q19<065401$$tNanotechnology$$v19$$x0957-4484$$y2008
000060999 8567_ $$uhttp://dx.doi.org/10.1088/0957-4484/19/6/065401
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000060999 9201_ $$0I:(DE-Juel1)VDB381$$d14.09.2008$$gCNI$$kCNI$$lCenter of Nanoelectronic Systems for Information Technology$$x1$$z381
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