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@ARTICLE{Hallquist:6250,
author = {Hallquist, M. and Wenger, J.C. and Baltensperger, U. and
Rudich, Y. and Simpson, D. and Claeys, M. and Dommen, J. and
Donahue, N.M. and George, C. and Goldstein, A.H. and
Hamilton, J.F. and Herrmann, H. and Hoffmann, T. and Iinuma,
Y. and Jang, M. and Jenkin, M. and Jimenez, J.L. and
Kiendler-Scharr, A. and Maenhaut, W. and McFiggans, G. and
Mentel, T. F. and Monod, A. and Prévôt, A.S.H. and
Seinfeld, J.H. and Surratt, J.D. and Szmigielski, R. and
Wildt, J.},
title = {{T}he formation, properties and impact of secondary organic
aerosol: current and emerging issues},
journal = {Atmospheric chemistry and physics},
volume = {9},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-6250},
pages = {5155 - 5235},
year = {2009},
note = {This review is the result of presentations and discussions
during the joint VOCBAS-INTROP conference on Biogenic
Volatile Organic Compounds: Sources and Fates in a
ChangingWorld. The authors would like to thank M. Staudt and
his colleagues at the Centre for Evolutionary and Functional
Ecology in Montpellier, France, for hosting the event.
Financial support from the European Science Foundation
INTROP programme is gratefully acknowledged. The authors
would also like to acknowledge funding received from; the
European Commission (EUROCHAMP, RII3-CT-2004-505968;
EUCAARI, 036833-2; POLYSOA, 12709; Marie Curie postdoctoral
fellowship to R. S.); European Monitoring and Evaluation
Programme (EMEP); the Swedish Research Council Formas
(contract 214-2006-1204); Science Foundation Ireland; the
Swiss National Science Foundation; the Israel Science
Foundation (grants 1527/07 and 196/08) and the Helen and
Martin Kimmel Award for Innovative Investigation; Belgian
Federal Science Policy Office (BIOSOL project); the Fund for
Scientific Research Flanders (FWO); DOE BER/ASP
(DEFG0208ER64627); the UK Department for Environment, Food
and Rural Affairs (contract AQ0704); NOAA OGP
(NA08OAR4310565); US EPA (STAR R833746, RD-83374901); DOE
(DEFG02-05ER63983); US National Science Foundation
(ATM-0703914).},
abstract = {Secondary organic aerosol (SOA) accounts for a significant
fraction of ambient tropospheric aerosol and a detailed
knowledge of the formation, properties and transformation of
SOA is therefore required to evaluate its impact on
atmospheric processes, climate and human health. The
chemical and physical processes associated with SOA
formation are complex and varied, and, despite considerable
progress in recent years, a quantitative and predictive
understanding of SOA formation does not exist and therefore
represents a major research challenge in atmospheric
science. This review begins with an update on the current
state of knowledge on the global SOA budget and is followed
by an overview of the atmospheric degradation mechanisms for
SOA precursors, gas-particle partitioning theory and the
analytical techniques used to determine the chemical
composition of SOA. A survey of recent laboratory, field and
modeling studies is also presented. The following topical
and emerging issues are highlighted and discussed in detail:
molecular characterization of biogenic SOA constituents,
condensed phase reactions and oligomerization, the
interaction of atmospheric organic components with sulfuric
acid, the chemical and photochemical processing of organics
in the atmospheric aqueous phase, aerosol formation from
real plant emissions, interaction of atmospheric organic
components with water, thermodynamics and mixtures in
atmospheric models. Finally, the major challenges ahead in
laboratory, field and modeling studies of SOA are discussed
and recommendations for future research directions are
proposed.},
keywords = {J (WoSType)},
cin = {ICG-2 / ICG-3},
ddc = {550},
cid = {I:(DE-Juel1)VDB791 / I:(DE-Juel1)ICG-3-20090406},
pnm = {Atmosphäre und Klima / Terrestrische Umwelt},
pid = {G:(DE-Juel1)FUEK406 / G:(DE-Juel1)FUEK407},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000268535500040},
url = {https://juser.fz-juelich.de/record/6250},
}