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000006270 0247_ $$2DOI$$a10.1021/jp8096814
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000006270 084__ $$2WoS$$aChemistry, Physical
000006270 084__ $$2WoS$$aPhysics, Atomic, Molecular & Chemical
000006270 1001_ $$0P:(DE-HGF)0$$aGriffiths, P.T.$$b0
000006270 245__ $$aReactive Uptake of N2O5 by Aerosols Containing Dicarboxylic Acids. Effect of Particle Phase, Composition and Nitrate Content
000006270 260__ $$aWashington, DC$$bSoc.$$c2009
000006270 300__ $$a5082 - 5090
000006270 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
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000006270 440_0 $$03693$$aJournal of Physical Chemistry A$$v113$$x1089-5639$$y17
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000006270 520__ $$aReactive uptake coefficients for loss of N(2)O(5) to micron-size aerosols containing oxalic malonic, succinic, and glutaric acids, and mixtures with ammonium hydrogen sulfate and ammonium sulfate, are presented. The uptake measurements were made using two different systems: atmospheric pressure laminar flow tube reactor (Cambridge) and the Large Indoor Aerosol Chamber at Forschungszentrum Juelich. Generally good agreement is observed for the data recorded using the two techniques. Measured uptake coefficients lie in the range 5 x 10(-4)-3 x 10(-2), dependent on relative humidity, on particle phase, and on particle composition. Uptake to solid particles is generally slow, with observed uptake coefficients less than 1 x 10(-3), while uptake to liquid particles is around an order of magnitude more efficient. These results are rationalized using a numerical model employing explicit treatment of both transport and chemistry. Our results indicate a modest effect of the dicarboxylic acids on uptake and confirm the strong effect of particle phase, liquid water content, and particulate nitrate concentrations.
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000006270 650_2 $$2MeSH$$aAerosols: chemistry
000006270 650_2 $$2MeSH$$aDicarboxylic Acids: chemistry
000006270 650_2 $$2MeSH$$aNitrates: chemistry
000006270 650_2 $$2MeSH$$aNitrogen Oxides: chemistry
000006270 650_2 $$2MeSH$$aParticle Size
000006270 650_2 $$2MeSH$$aSulfates: chemistry
000006270 650_7 $$00$$2NLM Chemicals$$aAerosols
000006270 650_7 $$00$$2NLM Chemicals$$aDicarboxylic Acids
000006270 650_7 $$00$$2NLM Chemicals$$aNitrates
000006270 650_7 $$00$$2NLM Chemicals$$aNitrogen Oxides
000006270 650_7 $$00$$2NLM Chemicals$$aSulfates
000006270 650_7 $$010102-03-1$$2NLM Chemicals$$anitrogen pentoxide
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000006270 7001_ $$0P:(DE-HGF)0$$aBadger, C.L.$$b1
000006270 7001_ $$0P:(DE-HGF)0$$aCox, R.A.$$b2
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000006270 7001_ $$0P:(DE-Juel1)VDB88401$$aHenk, H.H.$$b4$$uFZJ
000006270 7001_ $$0P:(DE-Juel1)16346$$aMentel, T. F.$$b5$$uFZJ
000006270 773__ $$0PERI:(DE-600)2006031-2$$a10.1021/jp8096814$$gVol. 113, p. 5082 - 5090$$p5082 - 5090$$q113<5082 - 5090$$tThe @journal of physical chemistry <Washington, DC> / A$$v113$$x1089-5639$$y2009
000006270 8567_ $$uhttp://dx.doi.org/10.1021/jp8096814
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