Home > Publications database > Reactive Uptake of N2O5 by Aerosols Containing Dicarboxylic Acids. Effect of Particle Phase, Composition and Nitrate Content > print

001     6270
005     20240709081805.0
024 7 _ |2 pmid
|a pmid:19385680
024 7 _ |2 DOI
|a 10.1021/jp8096814
024 7 _ |2 WOS
|a WOS:000265529800035
037 _ _ |a PreJuSER-6270
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Chemistry, Physical
084 _ _ |2 WoS
|a Physics, Atomic, Molecular & Chemical
100 1 _ |a Griffiths, P.T.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Reactive Uptake of N2O5 by Aerosols Containing Dicarboxylic Acids. Effect of Particle Phase, Composition and Nitrate Content
260 _ _ |a Washington, DC
|b Soc.
|c 2009
300 _ _ |a 5082 - 5090
336 7 _ |a Journal Article
|0 PUB:(DE-HGF)16
|2 PUB:(DE-HGF)
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
|0 0
|2 EndNote
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a article
|2 DRIVER
440 _ 0 |a Journal of Physical Chemistry A
|x 1089-5639
|0 3693
|y 17
|v 113
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a Reactive uptake coefficients for loss of N(2)O(5) to micron-size aerosols containing oxalic malonic, succinic, and glutaric acids, and mixtures with ammonium hydrogen sulfate and ammonium sulfate, are presented. The uptake measurements were made using two different systems: atmospheric pressure laminar flow tube reactor (Cambridge) and the Large Indoor Aerosol Chamber at Forschungszentrum Juelich. Generally good agreement is observed for the data recorded using the two techniques. Measured uptake coefficients lie in the range 5 x 10(-4)-3 x 10(-2), dependent on relative humidity, on particle phase, and on particle composition. Uptake to solid particles is generally slow, with observed uptake coefficients less than 1 x 10(-3), while uptake to liquid particles is around an order of magnitude more efficient. These results are rationalized using a numerical model employing explicit treatment of both transport and chemistry. Our results indicate a modest effect of the dicarboxylic acids on uptake and confirm the strong effect of particle phase, liquid water content, and particulate nitrate concentrations.
536 _ _ |a Atmosphäre und Klima
|c P22
|2 G:(DE-HGF)
|0 G:(DE-Juel1)FUEK406
|x 0
588 _ _ |a Dataset connected to Web of Science, Pubmed
650 _ 2 |2 MeSH
|a Aerosols: chemistry
650 _ 2 |2 MeSH
|a Dicarboxylic Acids: chemistry
650 _ 2 |2 MeSH
|a Nitrates: chemistry
650 _ 2 |2 MeSH
|a Nitrogen Oxides: chemistry
650 _ 2 |2 MeSH
|a Particle Size
650 _ 2 |2 MeSH
|a Sulfates: chemistry
650 _ 7 |0 0
|2 NLM Chemicals
|a Aerosols
650 _ 7 |0 0
|2 NLM Chemicals
|a Dicarboxylic Acids
650 _ 7 |0 0
|2 NLM Chemicals
|a Nitrates
650 _ 7 |0 0
|2 NLM Chemicals
|a Nitrogen Oxides
650 _ 7 |0 0
|2 NLM Chemicals
|a Sulfates
650 _ 7 |0 10102-03-1
|2 NLM Chemicals
|a nitrogen pentoxide
650 _ 7 |a J
|2 WoSType
700 1 _ |a Badger, C.L.
|b 1
|0 P:(DE-HGF)0
700 1 _ |a Cox, R.A.
|b 2
|0 P:(DE-HGF)0
700 1 _ |a Folkers, M.
|b 3
|u FZJ
|0 P:(DE-Juel1)VDB405
700 1 _ |a Henk, H.H.
|b 4
|u FZJ
|0 P:(DE-Juel1)VDB88401
700 1 _ |a Mentel, T. F.
|b 5
|u FZJ
|0 P:(DE-Juel1)16346
773 _ _ |a 10.1021/jp8096814
|g Vol. 113, p. 5082 - 5090
|p 5082 - 5090
|q 113<5082 - 5090
|0 PERI:(DE-600)2006031-2
|t The @journal of physical chemistry / A
|v 113
|y 2009
|x 1089-5639
856 7 _ |u http://dx.doi.org/10.1021/jp8096814
909 C O |o oai:juser.fz-juelich.de:6270
|p VDB
913 1 _ |k P22
|v Atmosphäre und Klima
|l Atmosphäre und Klima
|b Umwelt
|z fortgesetzt als P23
|0 G:(DE-Juel1)FUEK406
|x 0
914 1 _ |y 2009
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
920 1 _ |k ICG-2
|l Troposphäre
|d 30.09.2010
|g ICG
|0 I:(DE-Juel1)VDB791
|x 1
970 _ _ |a VDB:(DE-Juel1)114467
980 _ _ |a VDB
980 _ _ |a ConvertedRecord
980 _ _ |a journal
980 _ _ |a I:(DE-Juel1)IEK-8-20101013
980 _ _ |a UNRESTRICTED
981 _ _ |a I:(DE-Juel1)ICE-3-20101013
981 _ _ |a I:(DE-Juel1)IEK-8-20101013

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