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@ARTICLE{Hayashi:7382,
author = {Hayashi, M. and Ootsuka, Y. and Paulsson, M. and Persson,
B. N. J. and Ueba, H.},
title = {{L}ateral hopping of {CO} molecules on {P}t(111) surface by
femtosecond laser pulses},
journal = {Physical review / B},
volume = {80},
number = {24},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-7382},
pages = {245409},
year = {2009},
note = {We gratefully acknowledge J. G,dde and U. Hofer for showing
us their experimental data before publication and useful
discussions. We also thank M. Bonn and Ch. Frischkorm for
discussions and a critical reading of the manuscript. This
work was supported by the Grant-in-Aid for Scientific
Research B (Grant No. 18340085) from the Japan Society for
the Promotion of Science.},
abstract = {Theory of heat transfer between adsorbate vibrational
degrees of freedom and ultrafast laser heated hot electrons
including vibrational intermode coupling is applied to
calculate two-pulse correlation, laser fluence dependence
and time dependence of lateral hopping of CO molecules from
a step to terrace site on a stepped Pt (111) surface. The
intermode coupling is a key ingredient to describe
vibrational heating of the frustrated translation mode
responsible for the CO hopping. The calculated results are
in good agreement with the experimental results, especially
if we scale down the experimentally determined absorbed
fluence. It is found that CO hopping is induced by indirect
heating of the FT mode by the FR mode with a strong
frictional coupling to hot electrons.},
keywords = {J (WoSType)},
cin = {IFF-1},
ddc = {530},
cid = {I:(DE-Juel1)VDB781},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK414},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000273229200113},
doi = {10.1103/PhysRevB.80.245409},
url = {https://juser.fz-juelich.de/record/7382},
}