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@ARTICLE{Sinha:807742,
author = {Sinha, P. R. and Sahu, L. K. and Manchanda, R. K. and
Sheel, V. and Deushi, M. and Kajino, M. and Schultz, Martin
and Nagendra, N. and Kumar, P. and Trivedi, D. B. and Koli,
S. K. and Peshin, S. K. and Swamy, Y. V. and Tzanis, C. G.
and Sreenivasan, S.},
title = {{T}ransport of tropospheric and stratospheric ozone over
{I}ndia: {B}alloon-borne observations and modeling analysis},
journal = {Atmospheric environment},
volume = {131},
issn = {1352-2310},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2016-02160},
pages = {228 - 242},
year = {2016},
abstract = {This study describes the spatio-temporal variation of
vertical profiles of ozone (O3) measured by balloon-borne
ozonesondes over two tropical sites of Trivandrum (TVM) and
Hyderabad (HYD) in India from January 2009 to December 2010.
In the lower troposphere, the mixing ratios of O3 over HYD
(18–66 ppbv) were similar to TVM (18–65 ppbv). In the
free troposphere, the O3 mixing ratios over HYD were higher
than those over TVM throughout the year. In the tropical
tropopause layer (TTL) region (above 15 km), the mixing
ratios of O3 over TVM were higher (83–358 ppbv) compared
to those measured over HYD (89–216 ppbv). Prevailing of O3
laminae between about 14 and 17 km is seen for both sites
for most profiles. A strong seasonal variation of O3 is
observed in the lower stratosphere between 18 and 24 km over
TVM, however, it is not pronounced for HYD. Transport of air
masses from the biomass burning region of the central
Africa, Southeast Asia and the Indo Gangetic plains (IGP)
influenced and led to enhancements of lower and
mid-tropospheric O3 over HYD and TVM while, the isentropic
(325 K) potential vorticity (PV) at 100 hPa showed transport
of O3–rich air from the lower stratosphere to the upper
troposphere during winter and spring months over both sites.
The free tropospheric O3 mixing ratios (FT-O3; 0–4 km)
contribute substantially to the tropospheric column O3 (TCO)
with an annual average fraction of $30\%$ and reveal the
similar seasonal variations over HYD and TVM. The vertical
profiles of O3 obtained from the Monitoring Atmospheric
Composition and Climate - Interim Implementation (MACC-II)
reanalysis and the Meteorological Research
Institute-Chemistry Climate Model version 2 (MRI-CCM2) are
compared with the ozonesonde data over both sites. The
simulated magnitude, phase and vertical gradient of O3 from
both MRI-CCM2 and MACC-II are in good agreement with
measurements in the stratosphere while there are significant
differences in the tropospheric columns.},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243)},
pid = {G:(DE-HGF)POF3-243},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000372763400022},
doi = {10.1016/j.atmosenv.2016.02.001},
url = {https://juser.fz-juelich.de/record/807742},
}