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024 7 _ |a 10.1103/PhysRevB.92.245441
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100 1 _ |a Heisterkamp, F.
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245 _ _ |a Inhomogeneous nuclear spin polarization induced by helicity-modulated optical excitation of fluorine-bound electron spins in ZnSe
260 _ _ |a College Park, Md.
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520 _ _ |a Optically induced nuclear spin polarization in a fluorine-doped ZnSe epilayer is studied by time-resolved Kerr rotation using resonant excitation of donor-bound excitons. Excitation with helicity-modulated laser pulses results in a transverse nuclear spin polarization, which is detected as a change of the Larmor precession frequency of the donor-bound electron spins. The frequency shift in dependence on the transverse magnetic field exhibits a pronounced dispersion-like shape with resonances at the fields of nuclear magnetic resonance of the constituent zinc and selenium isotopes. It is studied as a function of external parameters, particularly of constant and radio frequency external magnetic fields. The width of the resonance and its shape indicate a strong spatial inhomogeneity of the nuclear spin polarization in the vicinity of a fluorine donor. A mechanism of optically induced nuclear spin polarization is suggested based on the concept of resonant nuclear spin cooling driven by the inhomogeneous Knight field of the donor-bound electron.
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542 _ _ |i 2015-12-28
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700 1 _ |a Greilich, A.
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700 1 _ |a Zhukov, E. A.
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700 1 _ |a Kirstein, E.
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700 1 _ |a Kazimierczuk, T.
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700 1 _ |a Korenev, V. L.
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700 1 _ |a Yugova, I. A.
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700 1 _ |a Yakovlev, D. R.
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773 _ _ |a 10.1103/PhysRevB.92.245441
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