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@ARTICLE{He:808780,
      author       = {He, Xin and Wang, Jun and Wang, Rui and Qiu, Bao and
                      Frielinghaus, Henrich and Niehoff, Philip and Liu, Haidong
                      and Stan, Marian Cristian and Paillard, Elie and Winter,
                      Martin and Li, Jie},
      title        = {{A} 3{D} porous {L}i-rich cathode material with an in situ
                      modified surface for high performance lithium ion batteries
                      with reduced voltage decay},
      journal      = {Journal of materials chemistry / A},
      volume       = {4},
      number       = {19},
      issn         = {2050-7496},
      address      = {London {[u.a.]},
      publisher    = {RSC},
      reportid     = {FZJ-2016-02396},
      pages        = {7230-7237},
      year         = {2016},
      abstract     = {High crystallinity Li-rich porous materials integrated with
                      an in situ formed surface containing carbonaceous compounds
                      are synthesized through a facile approach. The rationally
                      designed procedure involves the formation of a specific
                      morphology of a hydroxide precursor assisted by a self-made
                      template and subsequent high temperature treatment to obtain
                      a Li1.2Mn0.56Ni0.16Co0.08O2 target product. The porous
                      morphology is investigated using field-emission scanning
                      electron microscopy and its surface area is quantitatively
                      examined by gas sorption analysis coupled with the
                      Brunauer–Emmett–Teller method. The crystallinity is
                      characterized by X-ray diffraction and high-resolution
                      transmission electron microscopy. X-ray photoelectron
                      spectroscopy, CHN elemental analysis and small angle neutron
                      scattering confirm the presence of carbonaceous compounds in
                      the surface composition. The prepared material exhibits
                      superior discharge rate capability and excellent cycling
                      stability. It shows minor capacity loss after 100 cycles at
                      0.5C and retains $94.9\%$ of its initial capacity after 500
                      cycles at 2C. Even more notably, the “voltage decay”
                      during cycling is also significantly decreased. It has been
                      found that carbonaceous compounds play a critical role in
                      reducing the layered to spinel structural transformation
                      during cycling. Therefore, the present porous Li-rich
                      material with surface modified carbonaceous compounds
                      represents an attractive material for advanced lithium-ion
                      batteries.},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1 /
                      IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131) / 144 -
                      Controlling Collective States (POF3-144) / 6213 - Materials
                      and Processes for Energy and Transport Technologies
                      (POF3-621) / 6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich
                      Centre for Neutron Research (JCNS) (POF3-623)},
      pid          = {G:(DE-HGF)POF3-131 / G:(DE-HGF)POF3-144 /
                      G:(DE-HGF)POF3-6213 / G:(DE-HGF)POF3-6G15 /
                      G:(DE-HGF)POF3-6G4},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000376035300018},
      doi          = {10.1039/C6TA01448H},
      url          = {https://juser.fz-juelich.de/record/808780},
}