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000808812 1001_ $$0P:(DE-HGF)0$$aKlett, Joachim$$b0$$eCorresponding author
000808812 245__ $$aBand engineering for efficient catalyst-substrate coupling for photoelectrochemical water splitting
000808812 260__ $$aCambridge$$bRSC Publ.$$c2016
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000808812 520__ $$aTo achieve an overall efficient solar water splitting device, not only the efficiencies of photo-converter and catalyst are decisive, but also their appropriate coupling must be considered. In this report we explore the origin of a voltage loss occurring at the interface between a thin film amorphous silicon tandem cell and the TiO2 corrosion protection layer by means of XPS. We find that the overall device can be disassembled into its primary constituents and that they can be analyzed separately, giving insight into the device structure as a whole. Thus, a series of model experiments were conducted, each representing a part of the complete device. We finally arrive at the conclusion, that the formation of a SiO2 interfacial layer between the TiO2 protection layer and the silicon cell gives rise to the voltage loss observed for the whole device.
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000808812 536__ $$0G:(DE-Juel1)HITEC-20170406$$aHITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406)$$cHITEC-20170406$$x2
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000808812 7001_ $$0P:(DE-HGF)0$$aZiegler, Jürgen$$b1
000808812 7001_ $$0P:(DE-HGF)0$$aRadetinac, Aldin$$b2
000808812 7001_ $$0P:(DE-HGF)0$$aKaiser, Bernhard$$b3
000808812 7001_ $$0P:(DE-HGF)0$$aSchäfer, Rolf$$b4
000808812 7001_ $$0P:(DE-HGF)0$$aJaegermann, Wolfram$$b5
000808812 7001_ $$0P:(DE-Juel1)156469$$aUrbain, Félix$$b6$$ufzj
000808812 7001_ $$0P:(DE-Juel1)142337$$aBecker, Jan Philipp$$b7$$ufzj
000808812 7001_ $$0P:(DE-Juel1)130297$$aSmirnov, Vladimir$$b8$$ufzj
000808812 7001_ $$0P:(DE-Juel1)130238$$aFinger, Friedhelm$$b9$$ufzj
000808812 773__ $$0PERI:(DE-600)1476244-4$$a10.1039/C5CP06230F$$gVol. 18, no. 16, p. 10751 - 10757$$n16$$p10751 - 10757$$tPhysical chemistry, chemical physics$$v18$$x1463-9084$$y2016
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