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@ARTICLE{Klett:808812,
      author       = {Klett, Joachim and Ziegler, Jürgen and Radetinac, Aldin
                      and Kaiser, Bernhard and Schäfer, Rolf and Jaegermann,
                      Wolfram and Urbain, Félix and Becker, Jan Philipp and
                      Smirnov, Vladimir and Finger, Friedhelm},
      title        = {{B}and engineering for efficient catalyst-substrate
                      coupling for photoelectrochemical water splitting},
      journal      = {Physical chemistry, chemical physics},
      volume       = {18},
      number       = {16},
      issn         = {1463-9084},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {FZJ-2016-02427},
      pages        = {10751 - 10757},
      year         = {2016},
      abstract     = {To achieve an overall efficient solar water splitting
                      device, not only the efficiencies of photo-converter and
                      catalyst are decisive, but also their appropriate coupling
                      must be considered. In this report we explore the origin of
                      a voltage loss occurring at the interface between a thin
                      film amorphous silicon tandem cell and the TiO2 corrosion
                      protection layer by means of XPS. We find that the overall
                      device can be disassembled into its primary constituents and
                      that they can be analyzed separately, giving insight into
                      the device structure as a whole. Thus, a series of model
                      experiments were conducted, each representing a part of the
                      complete device. We finally arrive at the conclusion, that
                      the formation of a SiO2 interfacial layer between the TiO2
                      protection layer and the silicon cell gives rise to the
                      voltage loss observed for the whole device.},
      cin          = {IEK-5},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-5-20101013},
      pnm          = {126 - Solar Fuels (POF3-126) / 121 - Solar cells of the
                      next generation (POF3-121) / HITEC - Helmholtz
                      Interdisciplinary Doctoral Training in Energy and Climate
                      Research (HITEC) (HITEC-20170406)},
      pid          = {G:(DE-HGF)POF3-126 / G:(DE-HGF)POF3-121 /
                      G:(DE-Juel1)HITEC-20170406},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000374786300009},
      doi          = {10.1039/C5CP06230F},
      url          = {https://juser.fz-juelich.de/record/808812},
}