000809309 001__ 809309
000809309 005__ 20230217124357.0
000809309 0247_ $$2doi$$a10.1103/PhysRevE.93.052607
000809309 0247_ $$2ISSN$$a1063-651X
000809309 0247_ $$2ISSN$$a1095-3787
000809309 0247_ $$2ISSN$$a1539-3755
000809309 0247_ $$2ISSN$$a1550-2376
000809309 0247_ $$2ISSN$$a2470-0053
000809309 0247_ $$2Handle$$a2128/11192
000809309 0247_ $$2WOS$$aWOS:000376261600007
000809309 0247_ $$2altmetric$$aaltmetric:21828841
000809309 0247_ $$2pmid$$apmid:27300951
000809309 037__ $$aFZJ-2016-02533
000809309 082__ $$a530
000809309 1001_ $$0P:(DE-Juel1)130955$$aSchober, H. R.$$b0$$eCorresponding author$$ufzj
000809309 245__ $$aHeterogeneous diffusion, viscosity, and the Stokes-Einstein relation in binary liquids
000809309 260__ $$aCollege Park, Md.$$bAPS$$c2016
000809309 264_1 $$2Crossref$$3online$$bAmerican Physical Society (APS)$$c2016-05-16
000809309 264_1 $$2Crossref$$3print$$bAmerican Physical Society (APS)$$c2016-05-01
000809309 3367_ $$2DRIVER$$aarticle
000809309 3367_ $$2DataCite$$aOutput Types/Journal article
000809309 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1520523195_23721
000809309 3367_ $$2BibTeX$$aARTICLE
000809309 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000809309 3367_ $$00$$2EndNote$$aJournal Article
000809309 520__ $$aWe investigate the origin of the breakdown of the Stokes-Einstein relation (SER) between diffusivity and viscosity in undercooled melts. A binary Lennard-Jones system, as a model for a metallic melt, is studied by molecular dynamics. A weak breakdown at high temperatures can be understood from the collectivization of motion, seen in the isotope effect. The strong breakdown at lower temperatures is connected to an increase in dynamic heterogeneity. On relevant time scales some particles diffuse much faster than the average or than predicted by the SER. The van Hove self-correlation function allows one to unambiguously identify slow particles. Their diffusivity is even less than predicted by the SER. The time span of these particles being slow particles, before their first conversion to be a fast one, is larger than the decay time of the stress correlation. The contribution of the slow particles to the viscosity rises rapidly upon cooling. Not only the diffusion but also the viscosity shows a dynamically heterogeneous scenario. We can define a “slow” viscosity. The SER is recovered as the relation between slow diffusivity and slow viscosity.
000809309 536__ $$0G:(DE-HGF)POF3-144$$a144 - Controlling Collective States (POF3-144)$$cPOF3-144$$fPOF III$$x0
000809309 536__ $$0G:(DE-Juel1)jiff07_20140501$$aDynamik in Gläsern und unterkühlten Schmelzen und Flüssigkeiten (jiff07_20140501)$$cjiff07_20140501$$fDynamik in Gläsern und unterkühlten Schmelzen und Flüssigkeiten$$x1
000809309 542__ $$2Crossref$$i2016-05-16$$uhttp://link.aps.org/licenses/aps-default-license
000809309 588__ $$aDataset connected to CrossRef
000809309 7001_ $$0P:(DE-HGF)0$$aPeng, H. L.$$b1
000809309 77318 $$2Crossref$$3journal-article$$a10.1103/physreve.93.052607$$bAmerican Physical Society (APS)$$d2016-05-16$$n5$$p052607$$tPhysical Review E$$v93$$x2470-0045$$y2016
000809309 773__ $$0PERI:(DE-600)2844562-4$$a10.1103/PhysRevE.93.052607$$gVol. 93, no. 5, p. 052607$$n5$$p052607$$tPhysical review / E$$v93$$x2470-0045$$y2016
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.pdf$$yOpenAccess
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.gif?subformat=icon$$xicon$$yOpenAccess
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000809309 8564_ $$uhttps://juser.fz-juelich.de/record/809309/files/PhysRevE.93.052607.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000809309 909CO $$ooai:juser.fz-juelich.de:809309$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000809309 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130955$$aForschungszentrum Jülich$$b0$$kFZJ
000809309 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$aExternal Institute$$b1$$kExtern
000809309 9131_ $$0G:(DE-HGF)POF3-144$$1G:(DE-HGF)POF3-140$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lFuture Information Technology - Fundamentals, Novel Concepts and Energy Efficiency (FIT)$$vControlling Collective States$$x0
000809309 9141_ $$y2016
000809309 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000809309 915__ $$0LIC:(DE-HGF)APS-112012$$2HGFVOC$$aAmerican Physical Society Transfer of Copyright Agreement
000809309 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000809309 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000809309 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000809309 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000809309 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5
000809309 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000809309 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bPHYS REV E : 2014
000809309 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000809309 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz
000809309 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000809309 920__ $$lyes
000809309 9201_ $$0I:(DE-Juel1)PGI-2-20110106$$kPGI-2$$lTheoretische Nanoelektronik$$x0
000809309 9201_ $$0I:(DE-82)080012_20140620$$kJARA-HPC$$lJARA - HPC$$x1
000809309 980__ $$ajournal
000809309 980__ $$aVDB
000809309 980__ $$aI:(DE-Juel1)PGI-2-20110106
000809309 980__ $$aI:(DE-82)080012_20140620
000809309 980__ $$aUNRESTRICTED
000809309 9801_ $$aFullTexts
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1002/andp.19053220806
000809309 999C5 $$1U. Balucani$$2Crossref$$oU. Balucani Dynamics of the Liquid State 1994$$tDynamics of the Liquid State$$y1994
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1113/jphysiol.1982.sp014272
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/S0301-4622(01)00194-6
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1111/j.1365-246X.1988.tb01124.x
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1126/science.276.5316.1245
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1051/jphysrad:01934005010049700
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00319108908028445
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4775741
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.65.1595
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1007/BF01323572
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.469425
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/jp960968a
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.80.2630
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1625793
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.90.015901
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.104.195901
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.107.165902
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.47.479
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.57.R39
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.81.4648
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.58.3515
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.60.5714
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.63.036701
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1445747
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0953-8984/15/32/301
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.2192769
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.78.064208
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.3204063
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.83.224201
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4944081
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4723683
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4792356
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.4882066
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.91.134204
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0034-4885/55/3/001
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevA.31.980
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.449616
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0953-8984/20/37/373101
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/jp047763j
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.69.061205
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/13642819908223061
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1209/0295-5075/111/56008
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/RevModPhys.75.237
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.70.224209
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.51.4626
000809309 999C5 $$1M. P. Allen$$2Crossref$$oM. P. Allen Computer Simulation of Liquids 1987$$tComputer Simulation of Liquids$$y1987
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.1.138
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.65.1219
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.80.4919
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1063/1.1677258
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0022-3719/7/21/011
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00268978100102711
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.51.2026
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.62.597
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/S0038-1098(01)00219-8
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.59.811
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1016/0022-3093(93)90106-8
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1143/PTPS.126.67
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.80.2338
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.82.5064
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.83.051501
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRev.136.A405
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.85.4293
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.99.060604
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevE.74.061501
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.85.024204
000809309 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1021/jp0477147