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@ARTICLE{Sang:810538,
      author       = {Sang, X. F. and Gensch, I. and Kammer, B. and Khan, A. and
                      Kleist, E. and Laumer, W. and Schlag, P. and Schmitt,
                      Sebastian and Wildt, J. and Zhao, R. and Mungall, E. L. and
                      Abbatt, J. P. D. and Kiendler-Scharr, A.},
      title        = {{C}hemical stability of levoglucosan: {A}n isotopic
                      perspective},
      journal      = {Geophysical research letters},
      volume       = {43},
      number       = {10},
      issn         = {0094-8276},
      address      = {Hoboken, NJ},
      publisher    = {Wiley},
      reportid     = {FZJ-2016-03201},
      pages        = {5419 - 5424},
      year         = {2016},
      abstract     = {The chemical stability of levoglucosan was studied by
                      exploring its isotopic fractionation during the oxidation by
                      hydroxyl radicals. Aqueous solutions as well as mixed
                      (NH4)2SO4-levoglucosan particles were exposed to OH. In both
                      cases, samples experiencing different extents of processing
                      were isotopically analyzed by Thermal Desorption-Gas
                      Chromatography-Isotope Ratio Mass Spectrometry (TD-GC-IRMS).
                      From the dependence of levoglucosan δ13C and concentration
                      on the reaction extent, the kinetic isotope effect (KIE) of
                      the OH oxidation reactions was determined to be
                      1.00187±0.00027 and 1.00229±0.00018, respectively. Both
                      show good agreement within the uncertainty range. For the
                      heterogeneous oxidation of particulate levoglucosan by
                      gas-phase OH, a reaction rate constant of
                      (2.67±0.03)·10−12 cm3 molecule−1S−1 was derived. The
                      laboratory kinetic data, together with isotopic source and
                      ambient observations, give information on the extent of
                      aerosol chemical processing in the atmosphere.},
      cin          = {IEK-8 / IBG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013 / I:(DE-Juel1)IBG-2-20101118},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243) / HITEC - Helmholtz
                      Interdisciplinary Doctoral Training in Energy and Climate
                      Research (HITEC) (HITEC-20170406)},
      pid          = {G:(DE-HGF)POF3-243 / G:(DE-Juel1)HITEC-20170406},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000378347500091},
      doi          = {10.1002/2016GL069179},
      url          = {https://juser.fz-juelich.de/record/810538},
}