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100 1 _ |a Elumeeva, Karina
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245 _ _ |a A Simple Approach towards High-Performance Perovskite-Based Bifunctional Oxygen Electrocatalysts
260 _ _ |a Weinheim
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520 _ _ |a To accelerate the large-scale commercialization of electrochemical energy storage and conversion technologies through water splitting and regeneration in reversible fuel cells, cost-effective, highly efficient, and durable reversible oxygen electrodes are required. We report a comparatively simple approach to modify a group of oxygen-evolving perovskites based on lanthanum cobaltite into effective bifunctional systems through partial atom substitution, which, upon intermixing with nitrogen-doped carbon nanotubes, achieve remarkably low round-trip overvoltage of <850 mV in the electrocatalysis of oxygen reduction and oxygen evolution in an alkaline electrolyte, KOH (0.1 m). Besides the bifunctional electrocatalytic performance, the composite systems with a low Fe content possessed promising long-term stability.
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700 1 _ |a Yang, Fengkai
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700 1 _ |a Xia, Wei
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700 1 _ |a Muhler, Martin
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700 1 _ |a Schuhmann, Wolfgang
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