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@ARTICLE{Aquilante:811208,
author = {Aquilante, Francesco and Autschbach, Jochen and Carlson,
Rebecca K. and Chibotaru, Liviu F. and Delcey, Mickaël G.
and De Vico, Luca and Galván, Ignacio Fdez. and Ferré,
Nicolas and Frutos, Luis Manuel and Gagliardi, Laura and
Garavelli, Marco and Giussani, Angelo and Hoyer, Chad E. and
Li Manni, Giovanni and Lischka, Hans and Ma, Dongxia and
Malmqvist, Per Åke and Mueller, Thomas and Nenov, Artur and
Olivucci, Massimo and Pedersen, Thomas Bondo and Peng,
Daoling and Plasser, Felix and Pritchard, Ben and Reiher,
Markus and Rivalta, Ivan and Schapiro, Igor and
Segarra-Martí, Javier and Stenrup, Michael and Truhlar,
Donald G. and Ungur, Liviu and Valentini, Alessio and
Vancoillie, Steven and Veryazov, Valera and Vysotskiy,
Victor P. and Weingart, Oliver and Zapata, Felipe and Lindh,
Roland},
title = {{M}olcas 8: {N}ew capabilities for multiconfigurational
quantum chemical calculations across the periodic table},
journal = {Journal of computational chemistry},
volume = {37},
number = {5},
issn = {0192-8651},
address = {New York, NY [u.a.]},
publisher = {Wiley},
reportid = {FZJ-2016-03711},
pages = {506 - 541},
year = {2016},
abstract = {In this report, we summarize and describe the recent unique
updates and additions to the Molcas quantum chemistry
program suite as contained in release version 8. These
updates include natural and spin orbitals for studies of
magnetic properties, local and linear scaling methods for
the Douglas–Kroll–Hess transformation, the generalized
active space concept in MCSCF methods, a combination of
multiconfigurational wave functions with density functional
theory in the MC-PDFT method, additional methods for
computation of magnetic properties, methods for
diabatization, analytical gradients of state average
complete active space SCF in association with density
fitting, methods for constrained fragment optimization,
large-scale parallel multireference configuration
interaction including analytic gradients via the interface
to the Columbus package, and approximations of the CASPT2
method to be used for computations of large systems. In
addition, the report includes the description of a
computational machinery for nonlinear optical spectroscopy
through an interface to the QM/MM package Cobramm. Further,
a module to run molecular dynamics simulations is added, two
surface hopping algorithms are included to enable
nonadiabatic calculations, and the DQ method for
diabatization is added. Finally, we report on the subject of
improvements with respects to alternative file options and
parallelization.},
cin = {JSC},
ddc = {540},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {511 - Computational Science and Mathematical Methods
(POF3-511)},
pid = {G:(DE-HGF)POF3-511},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000369176900005},
pubmed = {pmid:26561362},
doi = {10.1002/jcc.24221},
url = {https://juser.fz-juelich.de/record/811208},
}