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@ARTICLE{Schweflinghaus:811255,
author = {Schweflinghaus, Benedikt and Zimmermann, Bernd and Heide,
M. and Bihlmayer, G. and Blügel, S.},
title = {{R}ole of {D}zyaloshinskii-{M}oriya interaction for
magnetism in transition-metal chains at {P}t step edges},
journal = {Physical review / B},
volume = {94},
number = {2},
issn = {2469-9950},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2016-03756},
pages = {024403},
year = {2016},
abstract = {We explore the emergence of chiral magnetism in
one-dimensional monatomic Mn, Fe, and Co chains deposited at
the Pt(664) step edge carrying out an ab initio study based
on density functional theory (DFT). The results are analyzed
employing several models: (i) a micromagnetic model, which
takes into account the Dzyaloshinskii-Moriya interaction
(DMI) besides the spin stiffness and the magnetic anisotropy
energy, and (ii) the Fert-Levy model of the DMI for diluted
magnetic impurities in metals. Due to the step-edge
geometry, the direction of the Dzyaloshinskii vector (D
vector) is not predetermined by symmetry and points in an
off-symmetry direction. For the Mn chain we predict a
long-period cycloidal spin-spiral ground state of unique
rotational sense on top of an otherwise atomic-scale
antiferromagnetic phase. The spins rotate in a plane that is
tilted relative to the Pt surface by 62∘ towards the upper
step of the surface. The Fe and Co chains show a
ferromagnetic ground state since the DMI is too weak to
overcome their respective magnetic anisotropy barriers. An
analysis of domain walls within the latter two systems
reveals a preference for a Bloch wall for the Fe chain and a
Néel wall of unique rotational sense for the Co chain in a
plane tilted by 29∘ towards the lower step. Although the
atomic structure is the same for all three systems, not only
the size but also the direction of their effective D vectors
differ from system to system. The latter is in contradiction
to the Fert-Levy model. Due to the considered step-edge
structure, this work provides also insight into the effect
of roughness on DMI at surfaces and interfaces of magnets.
Beyond the discussion of the monatomic chains we provide
general expressions relating ab initio results to realistic
model parameters that occur in a spin-lattice or in a
micromagnetic model. We prove that a planar homogeneous
spiral of classical spins with a given wave vector rotating
in a plane whose normal is parallel to the D vector is an
exact stationary state solution of a spin-lattice model for
a periodic solid that includes Heisenberg exchange and DMI.
In the vicinity of a collinear magnetic state, assuming that
the DMI is much smaller than the exchange interaction, the
curvature and slope of the stationary energy curve of the
spiral as a function of the wave vector provide directly the
values of the spin stiffness and the spiralization required
in micromagnetic models. The validity of the Fert-Levy model
for the evaluation of micromagnetic DMI parameters and for
the analysis of ab initio calculations is explored for
chains. The results suggest that some care has to be taken
when applying the model to infinite periodic one-dimensional
systems.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143) /
Magnetic Anisotropy of Metallic Layered Systems and
Nanostructures $(jiff13_20131101)$},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143 /
$G:(DE-Juel1)jiff13_20131101$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000378909700004},
doi = {10.1103/PhysRevB.94.024403},
url = {https://juser.fz-juelich.de/record/811255},
}