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@ARTICLE{DalMaso:811717,
      author       = {Dal Maso, M. and Liao, L. and Wildt, J. and
                      Kiendler-Scharr, A. and Kleist, E. and Tillmann, R. and
                      Sipilä, M. and Hakala, J. and Lehtipalo, K. and Ehn, M. and
                      Kerminen, V.-M. and Kulmala, M. and Worsnop, D. and Mentel,
                      T.},
      title        = {{A} chamber study of the influence of boreal {BVOC}
                      emissions and sulfuric acid on nanoparticle formation rates
                      at ambient concentrations},
      journal      = {Atmospheric chemistry and physics},
      volume       = {16},
      number       = {4},
      issn         = {1680-7324},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {FZJ-2016-04101},
      pages        = {1955 - 1970},
      year         = {2016},
      abstract     = {Aerosol formation from biogenic and anthropogenic precursor
                      trace gases in continental background areas affects climate
                      via altering the amount of available cloud condensation
                      nuclei. Significant uncertainty still exists regarding the
                      agents controlling the formation of aerosol nanoparticles.
                      We have performed experiments in the Jülich
                      plant–atmosphere simulation chamber with instrumentation
                      for the detection of sulfuric acid and nanoparticles, and
                      present the first simultaneous chamber observations of
                      nanoparticles, sulfuric acid, and realistic levels and
                      mixtures of biogenic volatile compounds (BVOCs). We present
                      direct laboratory observations of nanoparticle formation
                      from sulfuric acid and realistic BVOC precursor vapour
                      mixtures performed at atmospherically relevant concentration
                      levels. We directly measured particle formation rates
                      separately from particle growth rates. From this, we
                      established that in our experiments, the formation rate was
                      proportional to the product of sulfuric acid and biogenic
                      VOC emission strength. The formation rates were consistent
                      with a mechanism in which nucleating BVOC oxidation products
                      are rapidly formed and activate with sulfuric acid. The
                      growth rate of nanoparticles immediately after birth was
                      best correlated with estimated products resulting from BVOC
                      ozonolysis.},
      cin          = {IEK-8 / IBG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013 / I:(DE-Juel1)IBG-2-20101118},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000372971500007},
      doi          = {10.5194/acp-16-1955-2016},
      url          = {https://juser.fz-juelich.de/record/811717},
}