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@ARTICLE{Berkemeier:811718,
      author       = {Berkemeier, Thomas and Ammann, Markus and Mentel, Thomas F.
                      and Pöschl, Ulrich and Shiraiwa, Manabu},
      title        = {{O}rganic {N}itrate {C}ontribution to {N}ew {P}article
                      {F}ormation and {G}rowth in {S}econdary {O}rganic {A}erosols
                      from α-{P}inene {O}zonolysis},
      journal      = {Environmental science $\&$ technology},
      volume       = {50},
      number       = {12},
      issn         = {1520-5851},
      address      = {Columbus, Ohio},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2016-04102},
      pages        = {6334 - 6342},
      year         = {2016},
      abstract     = {The chemical kinetics of organic nitrate production during
                      new particle formation and growth of secondary organic
                      aerosols (SOA) were investigated using the short-lived
                      radioactive tracer 13N in flow-reactor studies of α-pinene
                      oxidation with ozone. Direct and quantitative measurements
                      of the nitrogen content indicate that organic nitrates
                      accounted for $∼40\%$ of SOA mass during initial particle
                      formation, decreasing to $∼15\%$ upon particle growth to
                      the accumulation-mode size range (>100 nm). Experiments with
                      OH scavengers and kinetic model results suggest that organic
                      peroxy radicals formed by α-pinene reacting with secondary
                      OH from ozonolysis are key intermediates in the organic
                      nitrate formation process. The direct reaction of α-pinene
                      with NO3 was found to be less important for particle-phase
                      organic nitrate formation. The nitrogen content of SOA
                      particles decreased slightly upon increase of relative
                      humidity up to $80\%.$ The experiments show a tight
                      correlation between organic nitrate content and SOA
                      particle-number concentrations, implying that the condensing
                      organic nitrates are among the extremely low volatility
                      organic compounds (ELVOC) that may play an important role in
                      the nucleation and growth of atmospheric nanoparticles.},
      cin          = {IEK-8},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000378469900027},
      pubmed       = {pmid:27219077},
      doi          = {10.1021/acs.est.6b00961},
      url          = {https://juser.fz-juelich.de/record/811718},
}