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000811869 1001_ $$0P:(DE-Juel1)4548$$aSchlag, Patrick$$b0$$eCorresponding author$$ufzj
000811869 245__ $$aAerosol source apportionment from 1-year measurements at the CESAR tower in Cabauw, the Netherlands
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000811869 520__ $$aIntensive measurements of submicron aerosol particles and their chemical composition were performed with an Aerosol Chemical Speciation Monitor (ACSM) at the Cabauw Experimental Site for Atmospheric Research (CESAR) in Cabauw, the Netherlands, sampling at 5 m height above ground. The campaign lasted nearly 1 year from July 2012 to June 2013 as part of the EU-FP7-ACTRIS project (Q-ACSM Network). Including equivalent black carbon an average particulate mass concentration of 9.50 µg m−3 was obtained during the whole campaign with dominant contributions from ammonium nitrate (45 %), organic aerosol (OA, 29 %), and ammonium sulfate (19 %). There were 12 exceedances of the World Health Organization (WHO) PM2.5 daily mean limit (25 µg m−3) observed at this rural site using PM1 instrumentation only. Ammonium nitrate and OA represented the largest contributors to total particulate matter during periods of exceedance.Source apportionment of OA was performed season-wise by positive matrix factorization (PMF) using the multilinear engine 2 (ME-2) controlled via the source finder (SoFi). Primary organic aerosols were attributed mainly to traffic (8–16 % contribution to total OA, averaged season-wise) and biomass burning (0–23 %). Secondary organic aerosols (SOAs, 61–84 %) dominated the organic fraction during the whole campaign, particularly on days with high mass loadings. A SOA factor which is attributed to humic-like substances (HULIS) was identified as a highly oxidized background aerosol in Cabauw. This shows the importance of atmospheric aging processes for aerosol concentration at this rural site. Due to the large secondary fraction, the reduction of particulate mass at this rural site is challenging on a local scale.
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000811869 536__ $$0G:(EU-Grant)262254$$aACTRIS - Aerosols, Clouds, and Trace gases Research Infrastructure Network (262254)$$c262254$$fFP7-INFRASTRUCTURES-2010-1$$x1
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000811869 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, Astrid$$b1$$ufzj
000811869 7001_ $$0P:(DE-HGF)0$$aBlom, Marcus Johannes$$b2
000811869 7001_ $$0P:(DE-HGF)0$$aCanonaco, Francesco$$b3
000811869 7001_ $$0P:(DE-HGF)0$$aHenzing, Jeroen Sebastiaan$$b4
000811869 7001_ $$0P:(DE-HGF)0$$aMoerman, Marcel$$b5
000811869 7001_ $$0P:(DE-HGF)0$$aPrévôt, André Stephan Henry$$b6
000811869 7001_ $$0P:(DE-HGF)0$$aHolzinger, Rupert$$b7
000811869 773__ $$0PERI:(DE-600)2069847-1$$a10.5194/acp-16-8831-2016$$gVol. 16, no. 14, p. 8831 - 8847$$n14$$p8831 - 8847$$tAtmospheric chemistry and physics$$v16$$x1680-7324$$y2016
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