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@ARTICLE{Dima:816,
      author       = {Dima, G. E. and Beltramo, G. L. and Koper, M. T. M.},
      title        = {{N}itrate reduction on single-crystal platinum electrodes},
      journal      = {Electrochimica acta},
      volume       = {50},
      issn         = {0013-4686},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {PreJuSER-816},
      pages        = {4318 - 4326},
      year         = {2005},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The structure sensitivity of the reduction of nitrate has
                      been studied on a series of single-crystal platinum
                      electrodes by cyclic voltammmetry and in situ FTIRAS in
                      sulfuric and perchloric acid solutions. The nitrate
                      reduction is a structure-sensitive reaction on
                      single-crystal platinum electrodes. However, this structure
                      sensitivity is essentially controlled by other species
                      (hydrogen, sulfate) that interact strongly with the
                      electrode surface rather than by a structure-sensitive
                      nitrate adsorption, dissociation or reduction.Voltammetric
                      and spectroscopic data point to adsorbed nitric oxide (NO)
                      as the main stable intermediate of the nitrate reduction to
                      ammonia. No evidence for the formation of N2O was found. On
                      surfaces with sufficiently wide (111) terraces in the
                      absence of specifically adsorbed sulfate, an oxidizable
                      nitrate reduction product is detected voltammetrically,
                      which may tentatively be attributed to the formation of a
                      small amount of hydroxylamine earlier during the
                      voltammetric scan. (C) 2005 Elsevier Ltd. All rights
                      reserved.},
      keywords     = {J (WoSType)},
      cin          = {ISG-4},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB421},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK242},
      shelfmark    = {Electrochemistry},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000231202800015},
      doi          = {10.1016/j.electacta.2005.02.093},
      url          = {https://juser.fz-juelich.de/record/816},
}