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@ARTICLE{BenitoAbascal:817670,
      author       = {Benito Abascal, M. and Bläsing, Marc and Ninomiya, Y. and
                      Müller, Michael},
      title        = {{I}nfluence of {S}team, {H}ydrogen {C}hloride and
                      {H}ydrogen {S}ulphide on the {R}elease and {C}ondensation of
                      {Z}inc in {G}asification},
      journal      = {Industrial $\&$ engineering chemistry research},
      volume       = {55},
      number       = {25},
      issn         = {0888-5885},
      address      = {Columbus, Ohio},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2016-04338},
      pages        = {6911–6921},
      year         = {2016},
      abstract     = {The aim of this work was to assess the influence of H2O,
                      HCl, and H2S on the condensation and release of zinc. The
                      condensation behavior of the zinc vapors was investigated in
                      a heated flow channel reactor housed in a furnace with a gas
                      cooling zone, where eight glass filters were placed on
                      different cooling stages. The metal species deposited in the
                      filters were determined by means of ion chromatography (IC)
                      and inductively coupled plasma optical emission spectroscopy
                      (ICP-OES). Experiments on the release of the inorganic
                      vapors were carried out in a heated flow channel reactor
                      coupled to a molecular beam mass spectrometer (MBMS). The
                      experiments were carried out under two typical gasification
                      conditions (H2/H2O/He or Ar) and atmospheric pressure with
                      50 and 500 ppmv of HCl and H2S. Hot gas analysis was done at
                      900, 800, 700, and 500 °C. The condensation experiments
                      showed that zinc condensed as ZnO, ZnCl2, and ZnS under the
                      conditions considered. The species detected in the gas phase
                      were Zn, ZnO, ZnCl2, and ZnS. The experimental results were
                      compared with Scheil–Gulliver cooling calculations carried
                      out with FactSage 6.3 software. This model was proven to be
                      an excellent tool for the prediction of the behavior of zinc
                      under gasification conditions. Furthermore, the global
                      kinetics of the condensation experiments was clarified with
                      the thermodynamic pseudoequilibrium model recently developed
                      by researchers of Chubu University (Japan). With this work,
                      not only a good understanding of the behavior of the zinc
                      under gasification conditions was obtained, but also the
                      finding and evidence of a powerful tool for predicting fast
                      and easily the behavior of trace metals under gasification
                      conditions.},
      cin          = {IEK-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-2-20101013},
      pnm          = {111 - Efficient and Flexible Power Plants (POF3-111)},
      pid          = {G:(DE-HGF)POF3-111},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000378984600003},
      doi          = {10.1021/acs.iecr.6b01637},
      url          = {https://juser.fz-juelich.de/record/817670},
}