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@ARTICLE{Doppler:817904,
author = {Doppler, M. C. and Fleig, J. and Bram, M. and Opitz, A. K.},
title = {{T}he {C}apacitance of {N}ickel {P}attern {E}lectrodes on
{Z}irconia {E}lectrolyte},
journal = {Journal of the Electrochemical Society},
volume = {163},
number = {10},
issn = {1945-7111},
address = {Pennington, NJ},
publisher = {Electrochemical Soc.},
reportid = {FZJ-2016-04502},
pages = {H1019 - H1025},
year = {2016},
abstract = {Micro-structured thin-film electrodes were employed to
investigate the capacitive behavior of nickel on
yttria-stabilized zirconia (YSZ) electrolytes by means of
electrochemical impedance spectroscopy. Electrodes with
different shapes and electrode areas clearly showed a linear
relationship between capacitance and the electrode area.
Electrostatic double layer models, however, could not
explain the observed area specific capacitance value of ca.
3 F/m². This fact, the characteristic voltage dependence
with a hysteresis, and the effect of H2S on the electrode
capacitance indicate substantial contributions of a chemical
capacitance. Possible types of chemical capacitance in the
system Ni(H2/H2O)/YSZ are discussed and an oxygen partial
pressure dependent mechanism change is suggested.},
cin = {IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {135 - Fuel Cells (POF3-135) / SOFC - Solid Oxide Fuel Cell
(SOFC-20140602)},
pid = {G:(DE-HGF)POF3-135 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000389150900121},
doi = {10.1149/2.0951610jes},
url = {https://juser.fz-juelich.de/record/817904},
}