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@ARTICLE{Beltramo:818,
author = {Beltramo, G. L. and Ibach, H. and Linke, U. and Giesen, M.},
title = {{D}etermination of the step dipole moment and the step line
tension on {A}g(001) electrodes},
journal = {Electrochimica acta},
volume = {53},
issn = {0013-4686},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {PreJuSER-818},
pages = {6818 - 6823},
year = {2008},
note = {Record converted from VDB: 12.11.2012},
abstract = {Using impedance spectroscopy, we determined the step dipole
moment and the potential dependence of the step line tension
of silver electrodes in contact with an electrolyte: (0 0 1)
and vicinal surfaces (1 1 n) with n = 5 7, 11 in 10 mM
ClO4--solutions were investigated. The step dipole moment is
determined from the shift of the potential of zero charge
(pzc) as a function of the Surface step density. The dipole
moment per step atom Was found to be 3.5 +/- 0.5 x 10(-3) e
angstrom. From the pzc and the potential dependence of the
capacitance curves, the potential dependence of the surface
tension of the vicinal Surfaces is determined. The line
tension of the steps is then calculated from the difference
between the Surface tensions of stepped (1 1 n) and the
nominally step-free (0 0 1) Surfaces. The results are
compared to a previous Study on Au(1 1 n) surfaces. For
gold, the step line tension decreases roughly linear with
potential, whereas a parabolic shape is observed for silver.
(c) 2008 Elsevier Ltd. All rights reserved.},
keywords = {J (WoSType)},
cin = {IBN-4},
ddc = {540},
cid = {I:(DE-Juel1)VDB802},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK414},
shelfmark = {Electrochemistry},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000258975400018},
doi = {10.1016/j.electacta.2008.01.032},
url = {https://juser.fz-juelich.de/record/818},
}