| 001 | 818387 | ||
| 005 | 20240619091210.0 | ||
| 024 | 7 | _ | |a 10.1021/acs.macromol.6b00931 |2 doi |
| 024 | 7 | _ | |a 0024-9297 |2 ISSN |
| 024 | 7 | _ | |a 1520-5835 |2 ISSN |
| 024 | 7 | _ | |a WOS:000379704000032 |2 WOS |
| 037 | _ | _ | |a FZJ-2016-04848 |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |a Arbe, Arantxa |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Role of Dynamic Asymmetry on the Collective Dynamics of Comblike Polymers: Insights from Neutron Spin-Echo Experiments and Coarse-Grained Molecular Dynamics Simulations |
| 260 | _ | _ | |a Washington, DC |c 2016 |b Soc. |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1478619533_18229 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a We investigate the collective dynamics of comblike polymers displaying nanosegregation in side groups and main-chain rich domains, where side groups and backbones are dynamically equivalent. Neutron spin-echo experiments on poly(alkylene oxide)s with increasing side-group length have been focused on the decay of inter- and intradomain correlations and are complemented with molecular dynamics simulations on a coarse-grained model. In general, a good qualitative agreement between simulation and experiment is found. The collective times at inter- and intradomain levels converge with decreasing temperature, implying a common glass transition, and separate at high temperatures, revealing an increasing role of connectivity. The features of collective relaxations—regarding stretching, characteristic time, and temperature dependence—are independent of branching. The standard stretching for side-group motions and the closeness of collective and self-motions show that the anomalies exhibited by dynamically asymmetric comblike macromolecules disappear. |
| 536 | _ | _ | |a 6215 - Soft Matter, Health and Life Sciences (POF3-621) |0 G:(DE-HGF)POF3-6215 |c POF3-621 |f POF III |x 0 |
| 536 | _ | _ | |0 G:(DE-HGF)POF3-6G15 |f POF III |x 1 |c POF3-6G15 |a 6G15 - FRM II / MLZ (POF3-6G15) |
| 588 | _ | _ | |a Dataset connected to CrossRef |
| 650 | 2 | 7 | |a Soft Condensed Matter |0 V:(DE-MLZ)SciArea-210 |2 V:(DE-HGF) |x 0 |
| 650 | 1 | 7 | |a Polymers, Soft Nano Particles and Proteins |0 V:(DE-MLZ)GC-1602-2016 |2 V:(DE-HGF) |x 0 |
| 693 | _ | _ | |a Forschungs-Neutronenquelle Heinz Maier-Leibnitz |e J-NSE: Neutron spin-echo spectrometer |f NL2ao |1 EXP:(DE-MLZ)FRMII-20140101 |0 EXP:(DE-MLZ)J-NSE-20140101 |5 EXP:(DE-MLZ)J-NSE-20140101 |6 EXP:(DE-MLZ)NL2ao-20140101 |x 0 |
| 700 | 1 | _ | |a Moreno, Angel J. |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Allgaier, J. |0 P:(DE-Juel1)130501 |b 2 |u fzj |
| 700 | 1 | _ | |a Ivanova, Oxana |0 P:(DE-Juel1)136923 |b 3 |u fzj |
| 700 | 1 | _ | |a Fouquet, Peter |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Colmenero, Juan |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Richter, Dieter |0 P:(DE-Juel1)130917 |b 6 |u fzj |
| 773 | _ | _ | |a 10.1021/acs.macromol.6b00931 |g Vol. 49, no. 13, p. 4989 - 5000 |0 PERI:(DE-600)1491942-4 |n 13 |p 4989 - 5000 |t Macromolecules |v 49 |y 2016 |x 1520-5835 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.pdf |y Restricted |
| 856 | 4 | _ | |x icon |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.gif?subformat=icon |y Restricted |
| 856 | 4 | _ | |x icon-1440 |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.jpg?subformat=icon-1440 |y Restricted |
| 856 | 4 | _ | |x icon-180 |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.jpg?subformat=icon-180 |y Restricted |
| 856 | 4 | _ | |x icon-640 |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.jpg?subformat=icon-640 |y Restricted |
| 856 | 4 | _ | |x pdfa |u https://juser.fz-juelich.de/record/818387/files/acs.macromol.6b00931.pdf?subformat=pdfa |y Restricted |
| 909 | C | O | |o oai:juser.fz-juelich.de:818387 |p VDB:MLZ |p VDB |
| 910 | 1 | _ | |a Forschungszentrum Jülich |0 I:(DE-588b)5008462-8 |k FZJ |b 2 |6 P:(DE-Juel1)130501 |
| 910 | 1 | _ | |a Forschungszentrum Jülich |0 I:(DE-588b)5008462-8 |k FZJ |b 3 |6 P:(DE-Juel1)136923 |
| 910 | 1 | _ | |a Forschungszentrum Jülich |0 I:(DE-588b)5008462-8 |k FZJ |b 6 |6 P:(DE-Juel1)130917 |
| 913 | 1 | _ | |a DE-HGF |b Forschungsbereich Materie |l Von Materie zu Materialien und Leben |1 G:(DE-HGF)POF3-620 |0 G:(DE-HGF)POF3-621 |2 G:(DE-HGF)POF3-600 |v In-house research on the structure, dynamics and function of matter |9 G:(DE-HGF)POF3-6215 |x 0 |4 G:(DE-HGF)POF |3 G:(DE-HGF)POF3 |
| 913 | 1 | _ | |a DE-HGF |9 G:(DE-HGF)POF3-6G15 |x 1 |4 G:(DE-HGF)POF |v FRM II / MLZ |1 G:(DE-HGF)POF3-6G0 |0 G:(DE-HGF)POF3-6G15 |3 G:(DE-HGF)POF3 |2 G:(DE-HGF)POF3-600 |b Forschungsbereich Materie |l Großgeräte: Materie |
| 914 | 1 | _ | |y 2016 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0200 |2 StatID |b SCOPUS |
| 915 | _ | _ | |a No Authors Fulltext |0 StatID:(DE-HGF)0550 |2 StatID |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0600 |2 StatID |b Ebsco Academic Search |
| 915 | _ | _ | |a JCR |0 StatID:(DE-HGF)0100 |2 StatID |b MACROMOLECULES : 2015 |
| 915 | _ | _ | |a IF >= 5 |0 StatID:(DE-HGF)9905 |2 StatID |b MACROMOLECULES : 2015 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0150 |2 StatID |b Web of Science Core Collection |
| 915 | _ | _ | |a WoS |0 StatID:(DE-HGF)0110 |2 StatID |b Science Citation Index |
| 915 | _ | _ | |a WoS |0 StatID:(DE-HGF)0111 |2 StatID |b Science Citation Index Expanded |
| 915 | _ | _ | |a Peer Review |0 StatID:(DE-HGF)0030 |2 StatID |b ASC |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)1150 |2 StatID |b Current Contents - Physical, Chemical and Earth Sciences |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0310 |2 StatID |b NCBI Molecular Biology Database |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0300 |2 StatID |b Medline |
| 915 | _ | _ | |a Nationallizenz |0 StatID:(DE-HGF)0420 |2 StatID |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0199 |2 StatID |b Thomson Reuters Master Journal List |
| 920 | 1 | _ | |0 I:(DE-Juel1)JCNS-FRM-II-20110218 |k JCNS (München) ; Jülich Centre for Neutron Science JCNS (München) ; JCNS-FRM-II |l JCNS-FRM-II |x 0 |
| 920 | 1 | _ | |0 I:(DE-Juel1)JCNS-1-20110106 |k Neutronenstreuung ; JCNS-1 |l Neutronenstreuung |x 1 |
| 980 | _ | _ | |a journal |
| 980 | _ | _ | |a VDB |
| 980 | _ | _ | |a UNRESTRICTED |
| 980 | _ | _ | |a I:(DE-Juel1)JCNS-FRM-II-20110218 |
| 980 | _ | _ | |a I:(DE-Juel1)JCNS-1-20110106 |
| Library | Collection | CLSMajor | CLSMinor | Language | Author |
|---|
guest ::